{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,3]],"date-time":"2026-09-03T01:21:36Z","timestamp":1788398496071,"version":"build-2803163510"},"reference-count":114,"publisher":"American Chemical Society (ACS)","issue":"26","license":[{"start":{"date-parts":[[2025,6,23]],"date-time":"2025-06-23T00:00:00Z","timestamp":1750636800000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by-nc-nd\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100020546","name":"Canada's Oil Sands Innovation Alliance","doi-asserted-by":"publisher","id":[{"id":"10.13039\/501100020546","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100000038","name":"Natural Sciences and Engineering Research Council of Canada","doi-asserted-by":"publisher","award":["NSERC AMA ALLRP 587268"],"award-info":[{"award-number":["NSERC AMA ALLRP 587268"]}],"id":[{"id":"10.13039\/501100000038","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100009192","name":"Alberta Innovates","doi-asserted-by":"publisher","id":[{"id":"10.13039\/501100009192","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2025,7,8]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>The increasing demand for advanced thin-film composite (TFC) membranes stems from the limitations of current commercial membranes, particularly their vulnerability to biofouling. In this study, novel silver-based metal-azolate frameworks (Ag-MAFs) were grown insitu on the surface of TFC reverse osmosis (RO) membranes. This functionalization resulted in a 45% increase in permeate flux without compromising salt rejection (97.6%) compared to pristine TFC membranes. The surface functionalization process is rapid, non-destructive, and employs eco-friendly solvents, silver salts, and amino-benzimidazole ligands, enabling repeatable modifications without affecting separation efficiency. The successful integration of Ag-MAFs onto the membrane surface was confirmed through comprehensive chemical characterization, including Fourier transform infrared (FTIR) spectroscopy, X-ray photoelectron spectroscopy (XPS), and energy dispersive X-ray (EDX) analysis. Notably, Ag-MAFs demonstrated strong stability, with no detectable leaching or detachment after 20 days of continuous water immersion. Morphological analysis using scanning electron microscopy (SEM) and confocal microscopy revealed that Ag-MAFs nanoparticles imparted robust antibacterial activity, reducing live bacterial populations by nearly 99%. Filtration tests showed that Ag-MAFs functionalized membranes exhibited superior fouling resistance and higher water recovery ratios than pristine membranes during a 10 h filtration cycle. This study presents a scalable and reproducible approach for developing advanced antibiofouling TFC membranes capable of long-term operation, eliminating the need for module disassembly and enhancing membrane longevity in practical applications.<\/jats:p>","DOI":"10.1021\/acsomega.5c02816","type":"journal-article","created":{"date-parts":[[2025,6,23]],"date-time":"2025-06-23T12:32:00Z","timestamp":1750681920000},"page":"28191-28209","source":"Crossref","is-referenced-by-count":5,"title":["Facile Epitaxial\nGrowth of Novel Nanoscale Ag-MAFs\non Reverse Osmosis Membranes: Enhancing Performance, Antibacterial\nActivity, and (Bio)fouling Resistance"],"prefix":"10.1021","volume":"10","author":[{"given":"Seyedeh\nFatemeh","family":"Seyedpour","sequence":"first","affiliation":[{"name":"University of Alberta , , 9211 116 Street NW , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]},{"name":"University of Alberta , , CW 405, Biological Sciences Bldg , , ,","place":["Edmonton, Alberta, Canada, T6G 2E9"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5532-6882","authenticated-orcid":true,"given":"Pooria","family":"Karami","sequence":"additional","affiliation":[{"name":"University of Alberta , , 9211 116 Street NW , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Saeed","family":"Khoshhal Salestan","sequence":"additional","affiliation":[{"name":"University of Alberta , , 9211 116 Street NW , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]},{"name":"Chalmers University of Technology , , ,","place":["Gothenburg, Sweden, 412 96"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7802-2686","authenticated-orcid":true,"given":"Sadegh","family":"Aghapour Aktij","sequence":"additional","affiliation":[{"name":"University of Alberta , , 9211 116 Street NW , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]},{"name":"University of Alberta , , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Upasana","family":"Singh","sequence":"additional","affiliation":[{"name":"University of Alberta , , CW 405, Biological Sciences Bldg , , ,","place":["Edmonton, Alberta, Canada, T6G 2E9"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Suyenna","family":"Huang","sequence":"additional","affiliation":[{"name":"University of Alberta , , CW 405, Biological Sciences Bldg , , ,","place":["Edmonton, Alberta, Canada, T6G 2E9"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6603-1649","authenticated-orcid":true,"given":"Jia Wei","family":"Chew","sequence":"additional","affiliation":[{"name":"Chalmers University of Technology , , ,","place":["Gothenburg, Sweden, 412 96"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0006-6658-9809","authenticated-orcid":true,"given":"Ahmad","family":"Rahimpour","sequence":"additional","affiliation":[{"name":"University of Alberta , , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3207-2434","authenticated-orcid":true,"given":"David","family":"Wishart","sequence":"additional","affiliation":[{"name":"University of Alberta , , CW 405, Biological Sciences Bldg , , ,","place":["Edmonton, Alberta, Canada, T6G 2E9"]},{"name":"University of Alberta , , 2-32 Athabasca Hall , , ,","place":["Edmonton, Alberta, Canada, T6G 2E8"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0403-8351","authenticated-orcid":true,"given":"Mohtada","family":"Sadrzadeh","sequence":"additional","affiliation":[{"name":"University of Alberta , , 9211 116 Street NW , , ,","place":["Edmonton, Alberta, Canada, T6G 1H9"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2025,6,23]]},"reference":[{"key":"2026081812070202800_cit1","doi-asserted-by":"crossref","first-page":"257","DOI":"10.1016\/B978-0-12-816710-6.00011-0","article-title":"Prospects of nanocomposite\nmembranes for water treatment by osmotic-driven membrane processes","volume-title":"Nanocomposite Membranes for Water and Gas Separation","author":"Khorshidi","year":"2020"},{"issue":"5","key":"2026081812070202800_cit2","doi-asserted-by":"publisher","first-page":"727","DOI":"10.1080\/00222338108056764","article-title":"Interfacial synthesis\nin the preparation of reverse osmosis membranes","volume":"15","author":"Cadotte","year":"1981","journal-title":"J. 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