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The nanoparticles (NP) preserved their crystalline magnetite structure after printing and calcium-mediated cross-linking, as confirmed by Fourier transform infrared spectroscopy (FTIR), X-ray diffraction (XRD), transmission electron microscopy (TEM), and thermogravimetric analysis (TGA). The printed hydrogels exhibited pH-responsive swelling behavior, with maximum hydration under acidic conditions. Adsorption experiments revealed that the formulation containing the highest NP loading achieved the greatest removal efficiency, reaching an adsorption capacity of 38.46 mg\u00b7g\u20131. Kinetic data were best described by the pseudo-second-order model, and equilibrium results followed the Langmuir isotherm, indicating monolayer adsorption governed by surface interactions. Overall, the combination of natural polymers, magnetic NP, and additive manufacturing provides a sustainable, efficient, and magnetically recoverable platform for the treatment of pesticide-contaminated water.<\/jats:p>","DOI":"10.1021\/acsomega.6c03353","type":"journal-article","created":{"date-parts":[[2026,8,7]],"date-time":"2026-08-07T20:01:53Z","timestamp":1786132913000},"page":"47866-47878","source":"Crossref","is-referenced-by-count":2,"title":["3D-Printed Magnetic\nPolysaccharide Hydrogels as Sustainable\nPlatforms for Pesticide Remediation"],"prefix":"10.1021","volume":"11","author":[{"given":"Yulianis P. Barraga\u0301n","family":"Medina","sequence":"first","affiliation":[{"name":"Instituto de Investigaciones en Ciencia y Tecnologi\u0301a de Materiales (INTEMA), CONICET-UNMdP , , Av. Colo\u0301n 10850 , , ,","place":["Mar del Plata, BA, Argentina, 7600"]},{"name":"Sa\u0303o Paulo State University (UNESP) , , Av. 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