{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,29]],"date-time":"2026-09-29T22:33:14Z","timestamp":1790721194366,"version":"4.1.0"},"reference-count":44,"publisher":"American Chemical Society (ACS)","issue":"35","license":[{"start":{"date-parts":[[2026,8,25]],"date-time":"2026-08-25T00:00:00Z","timestamp":1787616000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100012550","name":"Nemzeti Kutat?si, Fejleszt?si ls Innovaci?s Alap","doi-asserted-by":"publisher","award":["K135946"],"award-info":[{"award-number":["K135946"]}],"id":[{"id":"10.13039\/501100012550","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012550","name":"Nemzeti Kutat?si, Fejleszt?si ls Innovaci?s Alap","doi-asserted-by":"publisher","award":["RRF-2.3.1-21-2022-00009"],"award-info":[{"award-number":["RRF-2.3.1-21-2022-00009"]}],"id":[{"id":"10.13039\/501100012550","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,8]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Stabilizing lithium\u2013sulfur batteries in carbonate-based electrolytes requires simultaneous control over sulfur behavior and interfacial chemistry. In this work, we present a cooperative strategy that combines a poly(vinylidene fluoride) (PVDF)-derived ultramicroporous carbon (UMC) sulfur host with a 3,6-dioxa-1,8-octane-dithiol -poly(ethylene glycol) (DODT\u2013PEG) copolymer electrolyte additive to address these challenges in a unified manner. The ultramicroporous structure of UMC physically confines sulfur species within subnanometer pores, limiting polysulfide formation and outward diffusion, while the DODT\u2013PEG copolymer modifies the cathode\/electrolyte interphase to promote ion-conductive pathways and stabilize sulfur redox reactions. Through structural, electrochemical, impedance, and postmortem analyses, the distinct roles of sulfur confinement and interphase regulation are identified and correlated with improved electrochemical behavior. The combined system enables high reversible sulfur utilization, stable cycling with a Coulombic efficiency of &amp;gt;99%, and enhanced rate capability. Li\/\/Li symmetric cell analysis further reveals that the beneficial effect of the copolymer additive is localized at the cathode rather than at the lithium surface. This work demonstrates that coordinated host design and electrolyte engineering provide a simple and scalable route for improving Li\u2013S battery performance in conventional carbonate electrolytes.<\/jats:p>","DOI":"10.1021\/acsomega.6c06179","type":"journal-article","created":{"date-parts":[[2026,9,1]],"date-time":"2026-09-01T04:23:33Z","timestamp":1788236613000},"page":"53278-53290","source":"Crossref","is-referenced-by-count":2,"title":["Stabilizing Lithium\u2013Sulfur Batteries in Carbonate\nElectrolytes via DODT\u2013PEG Interphase Engineering and Ultramicroporous\nCarbon Confinement"],"prefix":"10.1021","volume":"11","author":[{"given":"Derek","family":"Ovc-Okene","sequence":"first","affiliation":[{"name":"HUN-REN Research Centre for Natural Sciences , , Magyar tudo\u0301sok krt. 2 , ,","place":["Budapest, Hungary, H-1117"]},{"name":"Budapest University of Technology and Economics , , Mu\u030begyetem rkp. 3 , ,","place":["Budapest, Hungary, H-1111"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lakshmi Shiva","family":"Shankar","sequence":"additional","affiliation":[{"name":"Zalaegerszeg Innovation Park, Sze\u0301chenyi Istva\u0301n University , Dr. Michelberger Pa\u0301l u\u0301t 3 , ,","place":["Zalaegerszeg, Hungary, H-8900"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pe\u0301ter","family":"Nagy","sequence":"additional","affiliation":[{"name":"University of Szeged , , Rerrich Be\u0301la te\u0301r 1 , ,","place":["Szeged, Hungary, H-6720"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Marton","family":"Szabados","sequence":"additional","affiliation":[{"name":"University of Szeged , , Rerrich Be\u0301la te\u0301r 1 , ,","place":["Szeged, Hungary, H-6720"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Da\u0301vid","family":"Ugi","sequence":"additional","affiliation":[{"name":"HUN-REN Research Centre for Natural Sciences , , Magyar tudo\u0301sok krt. 2 , ,","place":["Budapest, Hungary, H-1117"]},{"name":"Eo\u0308tvo\u0308s Lora\u0301nd University , , Pa\u0301zma\u0301ny Pe\u0301ter se\u0301tany 1\/a. , ,","place":["Budapest, Hungary, 1117"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"A\u0301kos","family":"Szabo\u0301","sequence":"additional","affiliation":[{"name":"HUN-REN Research Centre for Natural Sciences , , Magyar tudo\u0301sok Krt. 2 , ,","place":["Budapest, Hungary, H-1117"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2475-6841","authenticated-orcid":true,"given":"Be\u0301la","family":"Iva\u0301n","sequence":"additional","affiliation":[{"name":"HUN-REN Research Centre for Natural Sciences , , Magyar tudo\u0301sok Krt. 2 , ,","place":["Budapest, Hungary, H-1117"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5082-3422","authenticated-orcid":true,"given":"Robert","family":"Kun","sequence":"additional","affiliation":[{"name":"HUN-REN Research Centre for Natural Sciences , , Magyar tudo\u0301sok krt. 2 , ,","place":["Budapest, Hungary, H-1117"]},{"name":"Sze\u0301chenyi Istva\u0301n University , , Egyetem square 1 , ,","place":["Gyo\u030br, Hungary, H-9026"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,25]]},"reference":[{"key":"2026090809083900700_cit1","doi-asserted-by":"publisher","first-page":"A917","DOI":"10.1149\/2.0051706jes","article-title":"Electrodeposition kinetics in Li-S batteries: Effects\nof low electrolyte\/sulfur ratios and deposition surface composition","volume":"164","author":"Fan","year":"2017","journal-title":"J. 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