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[15]DBA produces a Trimer+Tetramer structure with a surprisingly large unit cell comprising 12 independent [15]DBA molecules. In contrast, [14]DBA forms a simple Dimer structure consisting of two [14]DBA molecules per unit cell. The lowest solute concentrations for SAMN formation are 2 \u00d7 10\u20136 mol\/L and 1 \u00d7 10\u20135 mol\/L for [14]DBA and [15]DBA, respectively, differing by approximately a factor of 5. Thus, even a slight modification of the triangular core shape leads to significant differences in their self-assembly behavior. Molecular mechanics (MM) simulations suggest that these differences arise, at least in part, from differences in intermolecular and molecule\u2013substrate interactions in SAMNs. Finally, mixing the constitutional isomers results in the formation of a regular coassembly, namely a Dimer+Dimer structure. The relative stabilities of the three structures are discussed based on experimental observations and nonbonding interactions estimated by MM simulations. This fundamental information is useful for advancing two-dimensional crystal engineering at the interface.<\/jats:p>","DOI":"10.1021\/acsomega.6c07826","type":"journal-article","created":{"date-parts":[[2026,9,3]],"date-time":"2026-09-03T19:43:26Z","timestamp":1788464606000},"page":"54689-54696","source":"Crossref","is-referenced-by-count":0,"title":["Self-Assembly of\nIsomeric Isosceles Triangle Molecules\nat the Liquid\u2013Solid Interface"],"prefix":"10.1021","volume":"11","author":[{"given":"Soto","family":"Moriya","sequence":"first","affiliation":[{"name":"Meiji University , , 1-1-1 Higashimita , Tama-ku, , ,","place":["Kawasaki, Kanagawa, Japan, 214-8571"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kazuya","family":"Sato","sequence":"additional","affiliation":[{"name":"Meiji University , , 1-1-1 Higashimita , Tama-ku, , ,","place":["Kawasaki, Kanagawa, Japan, 214-8571"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3634-541X","authenticated-orcid":true,"given":"Kazukuni","family":"Tahara","sequence":"additional","affiliation":[{"name":"Meiji University , , 1-1-1 Higashimita , Tama-ku, , ,","place":["Kawasaki, Kanagawa, Japan, 214-8571"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,9,3]]},"reference":[{"issue":"8","key":"2026091510092906900_cit1","doi-asserted-by":"publisher","first-page":"7445","DOI":"10.1021\/acsnano.8b03513","article-title":"Supramolecular Assemblies on Surfaces: Nanopatterning, Functionality,\nand Reactivity","volume":"12","author":"Goronzy","year":"2018","journal-title":"ACS Nano"},{"key":"2026091510092906900_cit2","doi-asserted-by":"publisher","first-page":"7298","DOI":"10.1002\/anie.200806339","article-title":"Molecular\nand Supramolecular Networks\non Surfaces: From Two-Dimensional Crystal Engineering to Reactivity","volume":"48","author":"Elemans","year":"2009","journal-title":"Angew. 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