{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T12:15:24Z","timestamp":1788524124740,"version":"build-2803163510"},"reference-count":48,"publisher":"American Chemical Society (ACS)","issue":"1","license":[{"start":{"date-parts":[[2019,1,7]],"date-time":"2019-01-07T00:00:00Z","timestamp":1546819200000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/pubs.acs.org\/page\/policy\/authorchoice_termsofuse.html"}],"funder":[{"DOI":"10.13039\/501100001501","name":"University Grants Commission","doi-asserted-by":"publisher","award":["2061410291"],"award-info":[{"award-number":["2061410291"]}],"id":[{"id":"10.13039\/501100001501","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001409","name":"Department of Science and Technology, Ministry of Science and Technology","doi-asserted-by":"publisher","award":["YSS\/2015\/000886"],"award-info":[{"award-number":["YSS\/2015\/000886"]}],"id":[{"id":"10.13039\/501100001409","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100008789","name":"Department of Science and Technology, Government of West Bengal","doi-asserted-by":"publisher","award":["113(Sanc.)\/ST\/P\/S&T\/15G-2\/2015"],"award-info":[{"award-number":["113(Sanc.)\/ST\/P\/S&T\/15G-2\/2015"]}],"id":[{"id":"10.13039\/501100008789","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2019,1,31]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>For initiating a prosperous cost-friendly waste management of small-scale industries, cow buffing dust (CBD), one of the abundantly available semisynthetic collagenic solid wastes, has been used as a nonsulfur cross-linker of natural rubber (NR) for fabricating an NRCBD\u2013biocomposite superadsorbent. The as-prepared reusable biocomposite bearing variegated collagenic and noncollagenic N-donors, along with the O-donors, has been reported for ligand-selective preferential superadsorption from waste water. Thus, a CBD and NR-based scalable biocomposite bearing optimum cross-linking, excellent physicochemical properties, and reusability has been developed via systematic optimization of the torque and reaction time for cost-friendly adsorptive exclusion of dyes, such as 2,8-dimethyl-3,7-diamino-phenazine (i.e., safranine, SF) and (7-amino-8-phenoxazin-3-ylidene)-diethylazanium dichlorozinc dichloride (i.e., brilliant cresyl blue), BCB, and Hg(II). The CBD-aided curing of NR has been achieved through the formation of a cross-linked chromane-ring originated via reaction between the methylol-phenol ring of phenol-formaldehyde resin and isoprene unit of NR. The partial disappearance of unsaturation in cured-NRCBD, relative variation of crystallinity, surface properties, elevated thermal stabilities, and ligand-selective superadsorption have been studied by advanced microstructural analyses of unadsorbed and\/or adsorbed NRCBD using Fourier transform infrared (FTIR), 13C nuclear magnetic resonance, ultraviolet\u2013visible, and O 1s-\/N 1s-\/C 1s-\/Hg 4f7\/2,5\/2-X-ray photoelectron spectroscopies, thermogravimetric analysis, differential scanning calorimetry, X-ray diffraction, field emission scanning electron microscopy, energy-dispersive spectroscopy, and pHPZC. Response surface methodology-based optimization has been employed to attain the optimum potential of NRCBD, considering the interactive effects between pHi, temperature, and concentration of the dye. H-aggregate and time-dependent hypochromic effect has been observed during individual adsorption of dyes. Moreover, the prevalence of chemisorption via ionic interaction between NRCBD and SF, BCB, and Hg(II) has been realized by FTIR, fitting of kinetics data to the pseudosecond-order model, and measurement of activation energies. The Brunauer\u2013Emmett\u2013Teller and Langmuir isotherms fit the best to BCB and SF\/Hg(II), respectively. Thermodynamically spontaneous chemisorption have shown the maximum adsorption capacities of 303.61, 46.14, and 166.46 mg g\u20131 for SF, BCB, and Hg(II), respectively, at low initial concentration of Hg(II)\/dyes = 40 ppm, 303 K, and adsorbent dose = 0.01 g.<\/jats:p>","DOI":"10.1021\/acsomega.8b02799","type":"journal-article","created":{"date-parts":[[2019,1,8]],"date-time":"2019-01-08T16:11:35Z","timestamp":1546963895000},"page":"421-436","source":"Crossref","is-referenced-by-count":34,"title":["Scalable Synthesis of Collagenic-Waste and Natural\nRubber-Based Biocomposite for Removal of Hg(II) and Dyes: Approach\nfor Cost-Friendly Waste Management"],"prefix":"10.1021","volume":"4","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-0219-1790","authenticated-orcid":true,"given":"Nayan Ranjan","family":"Singha","sequence":"first","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chandan","family":"Roy","sequence":"additional","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]},{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Manas","family":"Mahapatra","sequence":"additional","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Arnab","family":"Dutta","sequence":"additional","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Joy Sankar","family":"Deb Roy","sequence":"additional","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Madhushree","family":"Mitra","sequence":"additional","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pijush Kanti","family":"Chattopadhyay","sequence":"additional","affiliation":[{"name":"Maulana Abul Kalam Azad University of Technology , , Salt Lake, , ,","place":["Kolkata, West Bengal, India, 700106"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2019,1,7]]},"reference":[{"key":"2026090407151921200_cit1","doi-asserted-by":"publisher","first-page":"5776","DOI":"10.1021\/acssuschemeng.6b01760","article-title":"Turning\nVulcanized Natural Rubber\ninto a Self-Healing Polymer: Effect of the Disulfide\/Polysulfide Ratio","volume":"4","author":"Herna\u0301ndez","year":"2016","journal-title":"ACS Sustainable Chem. 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Interfaces"},{"key":"2026090407151921200_cit4","doi-asserted-by":"publisher","first-page":"5876","DOI":"10.1021\/ma800144u","article-title":"Comparative\nStudy on Strain-Induced Crystallization Behavior of Peroxide Cross-Linked\nand Sulfur Cross-Linked Natural Rubber","volume":"41","author":"Ikeda","year":"2008","journal-title":"Macromolecules"},{"key":"2026090407151921200_cit5","doi-asserted-by":"publisher","first-page":"735","DOI":"10.1002\/app.1994.070530603","article-title":"Vulcanization of Liquid Carboxyl-Terminated Rubber\nFilled with Leather Buffing Dust","volume":"53","author":"Kla\u0301sek","year":"1994","journal-title":"J. Appl. Polym.\nSci."},{"key":"2026090407151921200_cit6","doi-asserted-by":"publisher","first-page":"348","DOI":"10.1016\/j.jhazmat.2007.05.087","article-title":"Buffing Dust\nas a Filler of Carboxylated Butadiene-Acrylonitrile\nRubber and Butadiene-Acrylonitrile Rubber","volume":"151","author":"Chronska","year":"2008","journal-title":"J.\nHazard. Mater."},{"key":"2026090407151921200_cit7","doi-asserted-by":"publisher","first-page":"571","DOI":"10.1007\/s10098-014-0831-7","article-title":"Leather\nBoards from Buffing Dust: A Novel Perspective","volume":"17","author":"Senthil","year":"2014","journal-title":"Clean Technol. Environ. Policy"},{"key":"2026090407151921200_cit8","doi-asserted-by":"publisher","first-page":"1740","DOI":"10.1021\/ie034218g","article-title":"Removal of Rhodamine\nB, Fast Green, and Methylene Blue from Wastewater using Red Mud, an\nAluminum Industry Waste","volume":"43","author":"Gupta","year":"2004","journal-title":"Ind. Eng. Chem. Res."},{"key":"2026090407151921200_cit9","doi-asserted-by":"publisher","first-page":"326","DOI":"10.1021\/es071948x","article-title":"Human Exposure To Methylmercury through Rice Intake in Mercury Mining\nAreas, Guizhou Province, China","volume":"42","author":"Feng","year":"2008","journal-title":"Environ. 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