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Soc."},{"key":"ja075257cb00021\/ja075257cb00021_7","first-page":"1323","volume":"126","author":"Huang X.","year":"2004","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00022\/ja075257cb00022_1","first-page":"1312","volume":"1311","author":"Lipkowski P.","year":"1999","journal-title":"Chem. Commun."},{"key":"ja075257cb00023\/ja075257cb00023_1","doi-asserted-by":"crossref","first-page":"3908","DOI":"10.1021\/ja00063a008","volume":"115","author":"Ercolani G.","year":"1993","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00023\/ja075257cb00023_2","doi-asserted-by":"crossref","first-page":"5703","DOI":"10.1021\/jp9816723","volume":"102","author":"Ercolani G.","year":"1998","journal-title":"J. Phys. Chem. B"},{"key":"ja075257cb00023\/ja075257cb00023_3","first-page":"3818","volume":"34","author":"Sontjens S. H. M.","year":"2001","journal-title":"Macromolecules"},{"key":"ja075257cb00024\/ja075257cb00024_1","unstructured":"Despite well-resolved1H NMR spectra of these complexes, titration experiments could not be carried out in this solvent due to insufficient solubility of free1(\u22481.0 \u00d7 10-5M). For1\u00b7BM5\u22127, titration experiments were thus carried out under diluted conditions using UV\/Vis spectroscopy, affording well-defined binding isotherms indicative of 1:1 complexation with binding constantK> 108M-1(see Figure S6)."},{"key":"ja075257cb00026\/ja075257cb00026_1","doi-asserted-by":"crossref","first-page":"11139","DOI":"10.1021\/ja052645a","volume":"127","author":"Yagai S.","year":"2005","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00027\/ja075257cb00027_1","doi-asserted-by":"crossref","first-page":"7030","DOI":"10.1002\/anie.200602286","volume":"45","author":"Rosch U.","year":"2006","journal-title":"Angew. Chem., Int. Ed."},{"key":"ja075257cb00029\/ja075257cb00029_1","first-page":"1128","volume":"137","author":"Zhu W.","year":"2003","journal-title":"Synth. Met."},{"key":"ja075257cb00030\/ja075257cb00030_1","first-page":"1355","volume":"1354","author":"Ikeda M.","year":"2003","journal-title":"Chem. Commun."},{"key":"ja075257cb00031\/ja075257cb00031_1","doi-asserted-by":"crossref","first-page":"7394","DOI":"10.1002\/anie.200502316","volume":"44","author":"Xiao S.","year":"2005","journal-title":"Angew. Chem., Int. Ed."},{"key":"ja075257cb00032\/ja075257cb00032_1","doi-asserted-by":"crossref","first-page":"3037","DOI":"10.1021\/ja963687p","volume":"119","author":"Arehart S. V.","year":"1997","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00032\/ja075257cb00032_2","first-page":"272","volume":"30","author":"Hempenius M. A.","year":"1997","journal-title":"J. Macromolecules"},{"key":"ja075257cb00032\/ja075257cb00032_3","doi-asserted-by":"crossref","first-page":"1671","DOI":"10.1021\/ma010290j","volume":"35","author":"Busson P.","year":"2002","journal-title":"Macromolecules"},{"key":"ja075257cb00033\/ja075257cb00033_1","unstructured":"In decane, this complex (c= 2.0 \u00d7 10-3M) formed rigid gels upon aging for 1 month, indicating that polymerization occurs in this solvent. Similar solvent-induced polymerization has been reported for ureidopyrimidinone supramolecular polymers:\u2009 see ref 39d."},{"key":"ja075257cb00034\/ja075257cb00034_1","doi-asserted-by":"crossref","first-page":"2867","DOI":"10.1021\/ja00217a029","volume":"110","author":"Fuhrhop J. H.","year":"1988","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00035\/ja075257cb00035_1","first-page":"1384","volume":"1382","author":"Hanabusa K.","year":"1993","journal-title":"J. Chem. Soc., Chem. Commun."},{"key":"ja075257cb00036\/ja075257cb00036_1","first-page":"8653","volume":"122","author":"Jung J. H.","year":"2000","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00036\/ja075257cb00036_2","doi-asserted-by":"crossref","first-page":"7732","DOI":"10.1002\/anie.200602975","volume":"45","author":"Ajayaghosh A.","year":"2006","journal-title":"Angew. Chem., Int. Ed."},{"key":"ja075257cb00036\/ja075257cb00036_3","first-page":"6321","volume":"45","author":"Kumar N. S. S.","year":"2006","journal-title":"Angew. Chem., Int. Ed."},{"key":"ja075257cb00037\/ja075257cb00037_1","first-page":"8348","volume":"126","author":"Yao S.","year":"2004","journal-title":"J. Am. Chem. Soc."},{"key":"ja075257cb00039\/ja075257cb00039_1","doi-asserted-by":"crossref","first-page":"180","DOI":"10.1021\/ar960298r","volume":"31","author":"Gellman S. H.","year":"1998","journal-title":"Acc. Chem. Res."},{"key":"ja075257cb00039\/ja075257cb00039_2","first-page":"170","volume":"407","author":"Hirschberg J. H. K. K.","year":"2000","journal-title":"Nature"},{"key":"ja075257cb00039\/ja075257cb00039_3","first-page":"4011","volume":"101","author":"Hill D. J.","year":"2001","journal-title":"Chem. Rev."},{"key":"ja075257cb00039\/ja075257cb00039_4","first-page":"4231","volume":"9","author":"Hirschberg J. H. K. K.","year":"2003","journal-title":"Chem.Eur. J."},{"key":"ja075257cb00040\/ja075257cb00040_1","unstructured":"In our previous study, folding of supramolecular polymer chain was proposed for1\u00b7BM12from the UV\/Vis study:\u2009 the mixture showed a concentration-independent blue-shifted absorption band of1(\u03bbmax= 435 nm) above 2.5 \u00d7 10-4M (see refs 14b and 30b). The formation of H-type aggregates even in micromolar regime clearly demonstrates the intrachain stacking of1. In the present study, we found that1\u00b7BM11also shows similar H-aggregated band (\u03bbmax= 440 nm; see Table 1 and Figure S8) under the same concentration regime. In contrast, the formation of H-type aggregates is not observed for the columnar organization of the discrete 1 + 1 complexes of1\u00b7BM5\u22121\u00b7BM7where the disks can rotate freely around the column axis. For the folded supramolecular polymers of1\u00b7BM11\/12, rotational freedom of the constituent disks is restricted by the covalent linkers, and thereby the transition dipole moments of1within a column are locked in a specific orientation causing H-type exciton coupling."},{"key":"ja075257cb00041\/ja075257cb00041_1","doi-asserted-by":"crossref","first-page":"918","DOI":"10.1002\/anie.198909141","volume":"28","author":"Ringsdorf H.","year":"1989","journal-title":"Angew. Chem., Int. Ed."},{"key":"ja075257cb00041\/ja075257cb00041_2","doi-asserted-by":"crossref","first-page":"159","DOI":"10.1080\/02678299108036421","volume":"10","author":"Praefcke K.","year":"1991","journal-title":"Liq. Cryst."},{"key":"ja075257cb00041\/ja075257cb00041_3","first-page":"4342","volume":"33","author":"Kouwer P. H. J.","year":"2000","journal-title":"J. Macromolecules"}],"container-title":["Journal of the American Chemical Society"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/ja075257c","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2021,10,3]],"date-time":"2021-10-03T14:11:02Z","timestamp":1633270262000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/doi\/10.1021\/ja075257c"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2007,10,1]]},"references-count":122,"journal-issue":{"issue":"43","published-print":{"date-parts":[[2007,10,1]]}},"alternative-id":["10.1021\/ja075257c"],"URL":"https:\/\/doi.org\/10.1021\/ja075257c","relation":{},"ISSN":["0002-7863","1520-5126"],"issn-type":[{"value":"0002-7863","type":"print"},{"value":"1520-5126","type":"electronic"}],"subject":[],"published":{"date-parts":[[2007,10,1]]}}}