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Nevertheless, integrating antiferromagnets with semiconductors remains highly desirable to coordinate exciton emission, offering advantages of negligibly stray fields and faster spin dynamics. However, developing an effective approach to manipulate excitons via antiferromagnetic (AFM) magnons remains challenging. Here, we report magnon\u2013exciton coupling (MEC) in van der Waals (vdW) heterostructures and reveal the distinctive dependence of exciton emission on AFM spin order. Excitons selectively couple with Ne\u0301el-type antiferromagnets, resulting in a substantial increase in exciton energy. This is attributed to the formation of spin\u2013lattice-aligned channels that facilitate hopping-electron mediated magnon\u2013exciton interaction and valence band splitting. Our results pinpoint the essence of interlayer MEC with respect to AFM spin configuration, providing a new perspective for both elementary excitation modulation and the development of AFM-based opto-spintronics.<\/jats:p>","DOI":"10.1021\/jacs.6c04934","type":"journal-article","created":{"date-parts":[[2026,7,27]],"date-time":"2026-07-27T08:16:51Z","timestamp":1785140211000},"page":"31909-31917","source":"Crossref","is-referenced-by-count":0,"title":["Exciton Selectively\nCoupled to Magnon Dependent on\nSpin\u2013Lattice Alignment"],"prefix":"10.1021","volume":"148","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-0420-9461","authenticated-orcid":true,"given":"Chaocheng","family":"Liu","sequence":"first","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qi","family":"Jiang","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiyu","family":"Hu","sequence":"additional","affiliation":[{"name":"Hefei Normal University , , ,","place":["Hefei, China, 230601"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ruiqi","family":"Liu","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhi","family":"Li","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yafei","family":"Chu","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weican","family":"Lan","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ranran","family":"Zhang","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Hefei, China, 230031"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3378-6594","authenticated-orcid":true,"given":"Chao","family":"Wang","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hengli","family":"Duan","sequence":"additional","affiliation":[{"name":"Diamond Light Source , Harwell Science and Innovation Campus , ,","place":["Didcot, United Kingdom, OX11 0DE"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3298-4724","authenticated-orcid":true,"given":"Mao","family":"Ye","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences , , ,","place":["Shanghai, China, 201210"]},{"name":"Chinese Academy of Sciences , , ,","place":["Shanghai, China, 200050"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6297-4589","authenticated-orcid":true,"given":"Wensheng","family":"Yan","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , ,","place":["Hefei, China, 230026"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,27]]},"reference":[{"key":"2026080511132775800_cit1","doi-asserted-by":"publisher","first-page":"282","DOI":"10.1038\/s41586-022-05024-1","article-title":"Exciton-coupled coherent\nmagnons in a 2D semiconductor","volume":"609","author":"Bae","year":"2022","journal-title":"Nature"},{"key":"2026080511132775800_cit2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-024-47852-x","article-title":"Magnetically propagating\nHund\u2019s exciton in van der Waals antiferromagnet NiPS3","volume":"15","author":"He","year":"2024","journal-title":"Nat. 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