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Conventional catalytic methane combustion requires high temperatures (&amp;gt;400 \u00b0C) and is particularly inefficient at rather low concentrations (&amp;lt;1000 ppm). Herein, Pt\/CeO2 {111} nanocrystals assisted by photon-phonon codriven catalysis overcome these challenges. Ultrafast transient absorption spectroscopies confirm that CeO2 {111} efficiently harvests photons and promotes charge separation, while phonons promote the detrapping process and improve the initial charge separation, further enhancing the active charge populations. Meanwhile, Pt works as an efficient electron acceptor, enabling photohole oxidation of methane at the picosecond time scale and accelerating oxygen reduction reactions. All these results lead to a low light-off temperature T80 of 98 \u00b0C and a one-pass methane combustion efficiency of 95% with CO2 selectivity of near 100% at 200 \u00b0C, together with an apparent quantum efficiency of 36.5% and long-term stability over 100 h in the presence of even rather low methane concentrations of 500 ppm. These findings establish a scalable strategy for the efficient abatement of low-concentration methane emissions under mild conditions.<\/jats:p>","DOI":"10.1021\/jacs.6c05483","type":"journal-article","created":{"date-parts":[[2026,8,19]],"date-time":"2026-08-19T19:01:20Z","timestamp":1787166080000},"page":"36545-36554","source":"Crossref","is-referenced-by-count":0,"title":["Catalytic Combustion\nof Extremely Low Concentrations\nof Methane by Pt\/CeO2 {111} Nanocrystals Driven by the\nSynergy of Photons and Phonons"],"prefix":"10.1021","volume":"148","author":[{"given":"Chao","family":"Wang","sequence":"first","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]},{"name":"University College London , , ,","place":["London, U.K., WC1E 7JE"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Junjun","family":"Guo","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2963-9863","authenticated-orcid":true,"given":"Lunqiao","family":"Xiong","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiyi","family":"Li","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2629-9288","authenticated-orcid":true,"given":"Enqi","family":"Chen","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]},{"name":"University College London , , ,","place":["London, U.K., WC1E 7JE"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Youxun","family":"Xu","sequence":"additional","affiliation":[{"name":"University College London , , ,","place":["London, U.K., WC1E 7JE"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiarui","family":"Wu","sequence":"additional","affiliation":[{"name":"University College London , , ,","place":["London, U.K., WC1E 7JE"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Annika S.","family":"Tang","sequence":"additional","affiliation":[{"name":"University of Oxford , , ,","place":["Oxford, U.K., OX1 3PJ"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6231-9717","authenticated-orcid":true,"given":"Yang","family":"Lan","sequence":"additional","affiliation":[{"name":"University College London , , ,","place":["London, U.K., WC1E 7JE"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8885-1560","authenticated-orcid":true,"given":"Graham J.","family":"Hutchings","sequence":"additional","affiliation":[{"name":"Cardiff University , , ,","place":["Cardiff, U.K., CF24 4HQ"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2323-5510","authenticated-orcid":true,"given":"Junwang","family":"Tang","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, China, 100084"]},{"name":"University College London , , ,","place":["London, U.K., WC1E 7JE"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,19]]},"reference":[{"key":"2026090312095841000_cit1","volume-title":"Trends in globally-averaged\nCH4, N2O, and SF6 determined from\nNOAA Global Monitoring Laboratory measurements. 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