{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,19]],"date-time":"2026-08-19T15:26:15Z","timestamp":1787153175534,"version":"build-2736575974"},"reference-count":61,"publisher":"American Chemical Society (ACS)","issue":"32","license":[{"start":{"date-parts":[[2026,8,6]],"date-time":"2026-08-06T00:00:00Z","timestamp":1785974400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,8,6]],"date-time":"2026-08-06T00:00:00Z","timestamp":1785974400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,8,6]],"date-time":"2026-08-06T00:00:00Z","timestamp":1785974400000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China (NSFC)","doi-asserted-by":"crossref","award":["U21B2094"],"award-info":[{"award-number":["U21B2094"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,19]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Achieving precise control over ion and molecular transport under subnanometer confinement, especially beyond passive sieving, remains challenging in nanofluidics and membrane science. Here, we present a bioinspired strategy that enables the formation of subnanometer channels together with the integration of tunable molecular recognition within 2D amorphous polymer membranes. Large-area membranes with a size up to 900 cm2 were fabricated by interfacial cross-linking of supramolecular assemblies. Molecular-level control over the amphiphilicity of cucurbituril host\u2013guest complexes (HGCs) yields 1.6 nm thick amorphous monolayers with subnanometer pores at a high density of (1.5 \u00b1 0.5) \u00d7 1013 cm\u20132, comparable to that of covalent organic frameworks (COFs). The nanopores formed between cucurbituril hosts serve as dense transport pathways, while the intrinsic cavities act as dynamic host\u2013guest recognition sites. This architecture enables reversible charge-gating of ion transport via host\u2013guest recognition and delivers outstanding performance in osmotic power generation. This work provides a design strategy for constructing adaptive transport systems, introducing dynamic functionality into otherwise static porous architectures, with potential applications for responsive separation and advanced energy harvesting.<\/jats:p>","DOI":"10.1021\/jacs.6c07373","type":"journal-article","created":{"date-parts":[[2026,8,7]],"date-time":"2026-08-07T04:01:43Z","timestamp":1786075303000},"page":"34278-34288","source":"Crossref","is-referenced-by-count":0,"title":["Bioinspired Large-Area\nPolymeric Cucurbituril Monolayers\nwith Ultrahigh-Density Nanopores Enabling Reversible Charge-Gating\nof Ion Transport via Host\u2013Guest Recognition"],"prefix":"10.1021","volume":"148","author":[{"given":"Yehui","family":"Ding","sequence":"first","affiliation":[{"name":"Xi\u2019an Jiaotong University , , ,","place":["Xi\u2019an, China, 710049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-9167-0065","authenticated-orcid":true,"given":"Meng","family":"He","sequence":"additional","affiliation":[{"name":"Xi\u2019an Shiyou University , , ,","place":["Xi\u2019an, China, 710065"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianhui","family":"Lan","sequence":"additional","affiliation":[{"name":"Institute of High Energy Physics, Chinese Academy of Sciences , ,","place":["Beijing, China, 100049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fuzhu","family":"Liu","sequence":"additional","affiliation":[{"name":"Xi\u2019an Jiaotong University , , ,","place":["Xi\u2019an, China, 710049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3106-4061","authenticated-orcid":true,"given":"Dario","family":"Calvani","sequence":"additional","affiliation":[{"name":"Helmholtz-Zentrum Dresden-Rossendorf (HZDR) , , ,","place":["Go\u0308rlitz, Germany, 02826"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peng","family":"Lin","sequence":"additional","affiliation":[{"name":"China Nuclear Power Technology Research Institute Co., Ltd. , , ,","place":["Shenzhen, Guangdong, China, 518028"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yingzhe","family":"Du","sequence":"additional","affiliation":[{"name":"China Nuclear Power Technology Research Institute Co., Ltd. , , ,","place":["Shenzhen, Guangdong, China, 518028"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jun","family":"Sun","sequence":"additional","affiliation":[{"name":"Xi\u2019an Jiaotong University , , ,","place":["Xi\u2019an, China, 710049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiangdong","family":"Ding","sequence":"additional","affiliation":[{"name":"Xi\u2019an Jiaotong University , , ,","place":["Xi\u2019an, China, 710049"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9929-9732","authenticated-orcid":true,"given":"Weiqun","family":"Shi","sequence":"additional","affiliation":[{"name":"Shanghai Jiao Tong University , , ,","place":["Shanghai, China, 200240"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9723-4393","authenticated-orcid":true,"given":"Xue","family":"Liu","sequence":"additional","affiliation":[{"name":"Xi\u2019an Jiaotong University , , ,","place":["Xi\u2019an, China, 710049"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,6]]},"reference":[{"issue":"3","key":"2026081910244681500_cit1","doi-asserted-by":"publisher","first-page":"901","DOI":"10.1039\/B820556F","article-title":"Ion Transport\nin Nanofluidic Channels","volume":"39","author":"Daiguji","year":"2010","journal-title":"Chem. 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Funct.\nMater."},{"issue":"1","key":"2026081910244681500_cit25","doi-asserted-by":"publisher","first-page":"10666","DOI":"10.1038\/s41467-025-65691-2","article-title":"Polymorphic Functionalization Driven\nby Ion Displacement-Induced Antiferroelectric Ordering in CuBiP2Se6","volume":"16","author":"Yang","year":"2025","journal-title":"Nat. Commun."},{"issue":"50","key":"2026081910244681500_cit26","doi-asserted-by":"publisher","first-page":"46270","DOI":"10.1021\/jacs.5c15078","article-title":"A Funnel Diode Enabled by Nanopores-Decorated\nDielectric Polymer Monolayer for Integrated Field-Effect Gating, Rectification,\nand Memristive Switching","volume":"147","author":"Li","year":"2025","journal-title":"J. Am. Chem. 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Horiz."},{"issue":"3","key":"2026081910244681500_cit38","doi-asserted-by":"publisher","first-page":"381","DOI":"10.1002\/open.202000041","article-title":"Interfacial Synthesis of a Monolayered Fluorescent Two-Dimensional\nPolymer through Dynamic Imine Chemistry","volume":"9","author":"Zhang","year":"2020","journal-title":"ChemistryOpen"},{"issue":"1","key":"2026081910244681500_cit39","doi-asserted-by":"publisher","first-page":"305","DOI":"10.1146\/annurev.pc.46.100195.001513","article-title":"External Infrared Reflection Absorption\nSpectrometry of Monolayer Films at the Air-Water Interface","volume":"46","author":"Mendelsohn","year":"1995","journal-title":"Annu. Rev. Phys. Chem."},{"issue":"35","key":"2026081910244681500_cit40","doi-asserted-by":"publisher","first-page":"10429","DOI":"10.1039\/c0cp00071j","article-title":"Raman and SERS Spectroscopy\nof Cucurbit[n]urils","volume":"12","author":"Mahajan","year":"2010","journal-title":"Phys. Chem. Chem. 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