{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,7]],"date-time":"2026-08-07T14:22:22Z","timestamp":1786112542305,"version":"build-2736575974"},"reference-count":52,"publisher":"American Chemical Society (ACS)","issue":"30","license":[{"start":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T00:00:00Z","timestamp":1784592000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T00:00:00Z","timestamp":1784592000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T00:00:00Z","timestamp":1784592000000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52373005"],"award-info":[{"award-number":["52373005"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2022YFC2805103"],"award-info":[{"award-number":["2022YFC2805103"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100019793","name":"Guangdong Provincial Key Laboratory of Luminescence from Molecular Aggregates, South China University of Technology","doi-asserted-by":"publisher","award":["2023B1212060003"],"award-info":[{"award-number":["2023B1212060003"]}],"id":[{"id":"10.13039\/501100019793","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,5]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Amido groups are ubiquitous in natural and synthetic polymers and impart critical physiological and physicochemical properties. Conventional access to backbone-amido polymers, polyamides, generally relies on harsh conditions or highly reactive monomers to form amide bonds during polymerization. Here, we report a mild and atom-economic pathway to poly(ether amide)s (PEAs) through the linear step polymerization of diepoxides and amide-bearing primary diols formed in situ by amino alcohols, mostly derived from natural amino acids, and a reactive solvent, \u03b3-butyrolactone. The unique chemoselectivity of the Lewis pair (organo)catalyst enables preferential activation of primary hydroxyl groups toward epoxy ring opening in this multiprotonic system containing secondary\/tertiary hydroxyl and amido groups. The trimodular synthesis and abundant starting materials can be well-utilized for structural diversification and property refinement of PEAs, as showcased by their high interfacial performance in two divergent directions: (1) broad-spectrum protein resistance for the more hydrophilic ones, and (2) robust adhesion on various substrates even after 10 reuse cycles or at liquid nitrogen temperature, for the more hydrophobic ones.<\/jats:p>","DOI":"10.1021\/jacs.6c09368","type":"journal-article","created":{"date-parts":[[2026,7,21]],"date-time":"2026-07-21T20:04:45Z","timestamp":1784664285000},"page":"32473-32483","source":"Crossref","is-referenced-by-count":0,"title":["Site-Selective Trimodular\nPolymerization to Amino\nAcid-Based Poly(ether amide)s with Divergent Properties"],"prefix":"10.1021","volume":"148","author":[{"given":"Xingpei","family":"Hong","sequence":"first","affiliation":[{"name":"South China University of Technology , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0219-3729","authenticated-orcid":true,"given":"Guangzhao","family":"Zhang","sequence":"additional","affiliation":[{"name":"South China University of Technology , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2590-0027","authenticated-orcid":true,"given":"Junpeng","family":"Zhao","sequence":"additional","affiliation":[{"name":"South China University of Technology , , ,","place":["Guangzhou, China, 510640"]},{"name":"South China University of Technology , , ,","place":["Guangzhou, China, 510640"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,7,21]]},"reference":[{"issue":"7378","key":"2026080511132962800_cit1","doi-asserted-by":"publisher","first-page":"471","DOI":"10.1038\/nature10702","article-title":"Rethinking Amide Bond Synthesis","volume":"480","author":"Pattabiraman","year":"2011","journal-title":"Nature"},{"issue":"7","key":"2026080511132962800_cit2","doi-asserted-by":"publisher","DOI":"10.1002\/ange.202419978","article-title":"Polyglycidamides: From\nBackbone-Promoted Amidation to Degradable Polyether with Wide-Range\nLCST","volume":"137","author":"Hong","year":"2025","journal-title":"Angew. Chem."},{"issue":"51","key":"2026080511132962800_cit3","doi-asserted-by":"publisher","first-page":"15342","DOI":"10.1002\/anie.201506663","article-title":"Poly(N-isopropylacrylamide)\nPhase Diagrams: Fifty Years of Research","volume":"54","author":"Halperin","year":"2015","journal-title":"Angew.\nChem., Int. Ed."},{"issue":"1","key":"2026080511132962800_cit4","doi-asserted-by":"publisher","first-page":"22","DOI":"10.1002\/mren.201000017","article-title":"Polyamides\n\u2013 Still Strong after Seventy Years","volume":"5","author":"Marchildon","year":"2011","journal-title":"Macromol.\nReact. Eng."},{"issue":"11","key":"2026080511132962800_cit5","doi-asserted-by":"publisher","first-page":"5528","DOI":"10.1021\/cr900049t","article-title":"Synthesis\nof Well-Defined Polypeptide-Based Materials via the Ring-Opening Polymerization\nof \u03b1-Amino Acid N-Carboxyanhydrides","volume":"109","author":"Hadjichristidis","year":"2009","journal-title":"Chem. Rev."},{"issue":"14","key":"2026080511132962800_cit6","doi-asserted-by":"publisher","first-page":"4737","DOI":"10.1039\/C9CS00738E","article-title":"Ring Opening Polymerization of \u03b1-Amino Acids: Advances in Synthesis, Architecture and Applications\nof Polypeptides and Their Hybrids","volume":"49","author":"Rasines Mazo","year":"2020","journal-title":"Chem. Soc.\nRev."},{"issue":"3","key":"2026080511132962800_cit7","doi-asserted-by":"publisher","first-page":"936","DOI":"10.1021\/acs.biomac.7b01719","article-title":"Synthesis and Properties of Alternating Polypeptoids and Polyampholytes\nas Protein-Resistant Polymers","volume":"19","author":"Tao","year":"2018","journal-title":"Biomacromolecules"},{"issue":"5","key":"2026080511132962800_cit8","doi-asserted-by":"publisher","first-page":"1892","DOI":"10.1021\/acs.biomac.2c00150","article-title":"Recent Advances\nof Poly(ester amide)s-Based Biomaterials","volume":"23","author":"Han","year":"2022","journal-title":"Biomacromolecules"},{"issue":"7268","key":"2026080511132962800_cit9","doi-asserted-by":"publisher","first-page":"1234","DOI":"10.1038\/nature08403","article-title":"What Recent Ribosome Structures Have Revealed About\nthe Mechanism of Translation","volume":"461","author":"Schmeing","year":"2009","journal-title":"Nature"},{"issue":"25","key":"2026080511132962800_cit10","doi-asserted-by":"publisher","DOI":"10.1002\/ange.202505310","article-title":"Ring-Opening Polymerization Enables\nAccess to High-Performance Aliphatic-Aromatic Polyamides with Chemical\nRecyclability","volume":"137","author":"Tang","year":"2025","journal-title":"Angew. 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Mater."},{"issue":"8","key":"2026080511132962800_cit52","doi-asserted-by":"publisher","first-page":"972","DOI":"10.1021\/acsmacrolett.4c00383","article-title":"Polysquaramides","volume":"13","author":"Konar","year":"2024","journal-title":"ACS Macro Lett."}],"container-title":["Journal of the American\nChemical Society"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/jacs.6c09368","content-type":"application\/pdf","content-version":"vor","intended-application":"unspecified"},{"URL":"https:\/\/pubs.acs.org\/jacsat\/article-pdf\/148\/30\/32473\/66095534\/jacs.6c09368.pdf","content-type":"application\/pdf","content-version":"vor","intended-application":"syndication"},{"URL":"https:\/\/pubs.acs.org\/jacsat\/article-pdf\/148\/30\/32473\/66095534\/jacs.6c09368.pdf","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,8,5]],"date-time":"2026-08-05T15:14:29Z","timestamp":1785942869000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/jacsat\/article\/148\/30\/32473\/5225130\/Site-Selective-Trimodular-Polymerization-to-Amino"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,7,21]]},"references-count":52,"journal-issue":{"issue":"30","published-online":{"date-parts":[[2026,7,21]]},"published-print":{"date-parts":[[2026,8,5]]}},"URL":"https:\/\/doi.org\/10.1021\/jacs.6c09368","relation":{},"ISSN":["0002-7863","1520-5126"],"issn-type":[{"value":"0002-7863","type":"print"},{"value":"1520-5126","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,7,21]]}}}