{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,12]],"date-time":"2026-08-12T15:24:22Z","timestamp":1786548262001,"version":"build-2736575974"},"reference-count":61,"publisher":"American Chemical Society (ACS)","issue":"31","license":[{"start":{"date-parts":[[2026,8,2]],"date-time":"2026-08-02T00:00:00Z","timestamp":1785628800000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-029"},{"start":{"date-parts":[[2026,8,2]],"date-time":"2026-08-02T00:00:00Z","timestamp":1785628800000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-037"},{"start":{"date-parts":[[2026,8,2]],"date-time":"2026-08-02T00:00:00Z","timestamp":1785628800000},"content-version":"stm-asf","delay-in-days":0,"URL":"https:\/\/doi.org\/10.15223\/policy-045"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22475115"],"award-info":[{"award-number":["22475115"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,12]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>We report a tetrazine-regulated in situ hydrazine release strategy to synthesize highly crystalline azine-linked COFs (AZ-COFs) with varied central cores (triazine, cyanuric acid, benzene). The slow hydrolysis of 3,6-dimethyl-1,2,4,5-tetrazine enables controlled hydrazine generation, allowing kinetically moderated azine formation and overcoming crystallization challenges. The triazine-centered AZ-COF-1 exhibits enhanced charge separation and prolonged carrier lifetimes via efficient electronic coupling and dynamic conjugation switching, achieving an exceptionally high photocatalytic nicotinamide adenine dinucleotide (NADH) regeneration of 87.02% within 16 min. More importantly, the regenerated NADH can be directly coupled with l-glutamate dehydrogenase to drive the reductive amination of \u03b1-ketoglutarate, affording l-glutamic acid with high yield, thereby demonstrating its practical utility in photoenzymatic catalysis. This work not only establishes a simple and general strategy for the kinetically controlled synthesis of azine-linked COFs but also highlights the critical role of framework electronic structure in governing photocatalytic cofactor regeneration and downstream biotransformations, providing a promising platform for artificial photosynthesis and sustainable solar-to-chemical energy conversion.<\/jats:p>","DOI":"10.1021\/jacs.6c11128","type":"journal-article","created":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T14:37:53Z","timestamp":1785854273000},"page":"33757-33766","source":"Crossref","is-referenced-by-count":0,"title":["Tetrazine-Regulated\nSynthesis of Azine-Linked Covalent\nOrganic Frameworks for Photocatalytic Cofactor Regeneration and Photoenzymatic\nCatalysis"],"prefix":"10.1021","volume":"148","author":[{"given":"Xiudong","family":"Wang","sequence":"first","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhe","family":"Jiang","sequence":"additional","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jialin","family":"Cui","sequence":"additional","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fanqi","family":"Meng","sequence":"additional","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xuhan","family":"Zheng","sequence":"additional","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0714-9636","authenticated-orcid":true,"given":"Hui","family":"Liu","sequence":"additional","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2668-3722","authenticated-orcid":true,"given":"Yingjie","family":"Zhao","sequence":"additional","affiliation":[{"name":"Qingdao University of Science and Technology , , ,","place":["Qingdao, China, 266042"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,2]]},"reference":[{"issue":"5751","key":"2026081210075716200_cit1","doi-asserted-by":"publisher","first-page":"1166","DOI":"10.1126\/science.1120411","article-title":"Porous, crystalline, covalent organic\nframeworks","volume":"310","author":"Co\u0302te\u0301","year":"2005","journal-title":"Science"},{"issue":"17","key":"2026081210075716200_cit2","doi-asserted-by":"publisher","first-page":"6248","DOI":"10.1039\/D0CS00009D","article-title":"Chiral covalent organic frameworks: design, synthesis\nand property","volume":"49","author":"Han","year":"2020","journal-title":"Chem. 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