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Yet a few bulk chiral-structured superconductors are known, partly due to the difficulty in directly determining their atomic-scale chirality. Here, we report three chiral-structured superconductors, RhGe4, IrGe4, and IrSi4, synthesized under high pressure, with Tc values of \u223c2.6, 1.1, and 2.5 K, respectively. Using atomic-resolution Cs-corrected scanning transmission electron microscopy (STEM) combined with X-ray diffraction characterizations, we directly confirm their chiral structure (space group P3121). This real-space imaging approach overcomes ambiguities in traditional diffraction-based methods. These materials exhibit type-II superconductivity, and the enhancement of spin\u2013orbit coupling (SOC) leads to the emergence of mixed-parity pairing. Calculations also reveal symmetry-protected Weyl points near the Fermi level, which is robust against the SOC. Our work not only expands the family of chiral-structured superconductors but also demonstrates the indispensable role of STEM in directly determining chiral crystal structures. These materials thus offer a clean platform to explore the interplay among structural chirality, spin\u2013orbit coupling, mixed-parity superconductivity, and topological quantum phenomena.<\/jats:p>","DOI":"10.1021\/jacs.6c12142","type":"journal-article","created":{"date-parts":[[2026,8,4]],"date-time":"2026-08-04T13:11:24Z","timestamp":1785849084000},"page":"33970-33979","source":"Crossref","is-referenced-by-count":0,"title":["Chiral-Structured\nSuperconductors TrX4 (Tr\n= Rh, Ir; X = Ge, Si): A Platform for Mixed-Parity Pairing and Topological\nStates"],"prefix":"10.1021","volume":"148","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-6723-116X","authenticated-orcid":true,"given":"Zhenhai","family":"Yu","sequence":"first","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yunguan","family":"Ye","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , 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