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Herein, inspired by the growth of a two-dimensional (2D) perovskite layer, a class of aromatic organic cation ligands is adopted to stabilize CQDs and induce close and ordered packing of CQDs into a superlattice netted by an organic metal halogenide (QD@OMH), giving rise to a high carrier diffusion length (&amp;gt;250 nm) for lead sulfide (PbS) CQD film. The superlattice-based infrared photodetectors achieve a responsivity of 0.663 A W\u20131 at 1560 nm and an order-of-magnitude reduction in noise current density, yielding a detectivity exceeding 1013 Jones. Furthermore, the infrared light-emitting diodes achieve a high radiance (22.4 W sr\u20131 m\u20132) and an operational T90 lifetime exceeding 200 h under continuous operation at peak luminance.<\/jats:p>","DOI":"10.1021\/jacs.6c12708","type":"journal-article","created":{"date-parts":[[2026,8,14]],"date-time":"2026-08-14T14:02:26Z","timestamp":1786716146000},"page":"37318-37329","source":"Crossref","is-referenced-by-count":0,"title":["Organic\nMetal Halogenide Netted Colloidal Quantum\nDot Superlattice"],"prefix":"10.1021","volume":"148","author":[{"given":"Haobo","family":"Wu","sequence":"first","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu","family":"Chen","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0000-8840-0014","authenticated-orcid":true,"given":"Xin","family":"Wen","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weixuan","family":"Liu","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5520-0462","authenticated-orcid":true,"given":"Wenjia","family":"Zhou","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiahui","family":"Du","sequence":"additional","affiliation":[{"name":"University of Science and Technology of China , , , ,","place":["Hefei, Anhui, China, 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201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3443-8604","authenticated-orcid":true,"given":"Hao","family":"Wang","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Lu","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziyao","family":"Ma","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 201210"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yaxin","family":"Zhao","sequence":"additional","affiliation":[{"name":"ShanghaiTech University , , ,","place":["Shanghai, China, 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