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Among these properties, optical magneto-chiral anisotropy, the nonreciprocal absorption of light shown by chiral magnetized systems, is emerging as an enabling technology in magneto-optics and photonics. Here, we report on enantiopure chiral molecular crystals based on the erbium(III) rare-earth ion that display nonreciprocal, wavelength-selective, magnetic field-induced variations of the optical absorption coefficients up to ca. 200% for the intrashell f\u2013f electronic transition falling in the 1.5 \u03bcm telecom wavelength range. Such a response is associated with an exceptionally high Magneto-Chiral Dichroism induced by the strong spin\u2013orbit coupling of the Er(III) and the helical chirality at the lanthanide center, exalted by the magnetic-dipole-allowed character of the electronic transition. This chirality-induced nonreciprocal magneto-optical response represents a proof of concept for the use of these chiral crystalline molecular materials as potential components in magneto-optical diodes.<\/jats:p>","DOI":"10.1021\/jacs.6c14062","type":"journal-article","created":{"date-parts":[[2026,10,11]],"date-time":"2026-10-11T15:01:24Z","timestamp":1791730884000},"page":"44719-44729","source":"Crossref","is-referenced-by-count":0,"title":["Wavelength-Selective\nMagneto-Optical Diodes Based\non Rare-Earth Chiral Molecular Crystals"],"prefix":"10.1021","volume":"148","author":[{"given":"Inkarat","family":"Atirojwanich","sequence":"first","affiliation":[{"name":"CNRS, Univ. Grenoble Alpes, INSA Toulouse, Univ. Toulouse Paul Sabatier, EMFL , , ,","place":["Grenoble, France, 38042"]},{"name":"Univ Rennes, CNRS, ISCR (Institut des Sciences Chimiques de Rennes)-UMR 6226 , ,","place":["Rennes, France, F-35000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8808-5552","authenticated-orcid":true,"given":"Maxime","family":"Aragon-Alberti","sequence":"additional","affiliation":[{"name":"CNRS, Univ. Grenoble Alpes, INSA Toulouse, Univ. Toulouse Paul Sabatier, EMFL , , ,","place":["Grenoble, France, 38042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Langit Cahya","family":"Adi","sequence":"additional","affiliation":[{"name":"CNRS, Univ. Grenoble Alpes, INSA Toulouse, Univ. Toulouse Paul Sabatier, EMFL , , ,","place":["Grenoble, France, 38042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kevin","family":"Paillot","sequence":"additional","affiliation":[{"name":"CNRS, Univ. Grenoble Alpes, INSA Toulouse, Univ. Toulouse Paul Sabatier, EMFL , , ,","place":["Grenoble, France, 38042"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mathieu","family":"Gascoin","sequence":"additional","affiliation":[{"name":"Univ Rennes, CNRS, ISCR (Institut des Sciences Chimiques de Rennes)-UMR 6226 , ,","place":["Rennes, France, F-35000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9533-8765","authenticated-orcid":true,"given":"Gre\u0301goire","family":"David","sequence":"additional","affiliation":[{"name":"Univ Rennes, CNRS, ISCR (Institut des Sciences Chimiques de Rennes)-UMR 6226 , ,","place":["Rennes, France, F-35000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3013-0546","authenticated-orcid":true,"given":"Boris","family":"Le Guennic","sequence":"additional","affiliation":[{"name":"Univ Rennes, CNRS, ISCR (Institut des Sciences Chimiques de Rennes)-UMR 6226 , ,","place":["Rennes, France, F-35000"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2008-7943","authenticated-orcid":true,"given":"Geert L. 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J."},{"key":"2026102111073289500_cit25","doi-asserted-by":"publisher","first-page":"2806","DOI":"10.1021\/ic50211a063","article-title":"Selection\nrules for lanthanide optical activity","volume":"19","author":"Richardson","year":"1980","journal-title":"Inorg.\nChem."},{"key":"2026102111073289500_cit26","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202412521","article-title":"Magneto-Chiral Dichroism\nof Chiral Lanthanide Complexes in the Context\nof Richardson\u2019s Theory of Optical Activity","volume":"63","author":"Adi","year":"2024","journal-title":"Angew. Chem., Int. Ed."},{"key":"2026102111073289500_cit27","doi-asserted-by":"publisher","first-page":"67","DOI":"10.1021\/jacs.5c17544","article-title":"Magneto-Optical Readout of a Chiral Single-Molecule Magnet at Telecom\nWavelengths","volume":"148","author":"Aragon-Alberti","year":"2026","journal-title":"J. Am. Chem. 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In  Proceedings\nof the NATO Advanced Study Institute Held at the University of Sussex,\nFalmer, England, September 10\u201322, 1978; Springer Netherlands, 1979.","DOI":"10.1007\/978-94-015-7644-4"},{"key":"2026102111073289500_cit36","doi-asserted-by":"publisher","first-page":"2671","DOI":"10.1021\/jacs.0c13180","article-title":"Helicene-Based Ligands Enable Strong Magneto-Chiral\nDichroism in\na Chiral Ytterbium Complex","volume":"143","author":"Atzori","year":"2021","journal-title":"J. Am. Chem. 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Mater."},{"key":"2026102111073289500_cit52","doi-asserted-by":"publisher","first-page":"4016","DOI":"10.1039\/D5MH00192G","article-title":"Enlightening\nmolecular logic: basics, tools and techniques for newcomers","volume":"12","author":"Brites","year":"2025","journal-title":"Mater. Horiz."},{"key":"2026102111073289500_cit53","doi-asserted-by":"publisher","first-page":"453","DOI":"10.1107\/S002188980600731X","article-title":"Mercury:\nvisualization and analysis of crystal structures","volume":"39","author":"Macrae","year":"2006","journal-title":"J. Appl. Crystallogr."},{"key":"2026102111073289500_cit54","doi-asserted-by":"publisher","first-page":"532","DOI":"10.1021\/ed085p532","article-title":"Diamagnetic Corrections\nand Pascal\u2019s Constants","volume":"85","author":"Bain","year":"2008","journal-title":"J. Chem. 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