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However, precise control of their motion is still difficult because creating required asymmetric nanostructures presents significant synthetic challenges. Inspired by automotive engine control, this study reports a general strategy for constructing optical nanomotors with programmable motion. For the first time, this approach implements a \u201cGo and Stop\u201d concept, leveraging dissimilar near-infrared (NIR) responsivities of upconversion nanoparticle (UCNP) to accelerate (\u201cGo\u201d) or brake (\u201cStop\u201d) motion on demand. Specifically, the nanovehicle is designed via interface-guided anisotropic growth strategy, where half of a single upconversion nanoparticle (UCNP) is coated with a hydrophilic silica shell containing Au nanoseeds, while the other is covered by a hydrophobic periodic mesoporous organosilica (PMO) loaded with Roussin\u2019s black salt (RBS). This dual hydrophilic\/hydrophobic design is also applicable to other optical materials, thus demonstrating great flexibility. When excited at 980 nm, blue light emitted by the UCNP activates the RBS to release nitric oxide (NO), propelling the nanomotor forward. Conversely, light at 808 nm induces gold-mediated thermophoresis, which reduces and eventually stops NO-driven motion. Such \u201cpull\u2013push\u201d effect enables the nanomotor to start, accelerate, decelerate, and stop simply by switching the excitation light. As a proof of concept, the nanovehicle is further used to noninvasively regulate cellular endocytosis and has demonstrated great potentials for programmable tumor treatment.<\/jats:p>","DOI":"10.1021\/jacsau.6c00299","type":"journal-article","created":{"date-parts":[[2026,8,19]],"date-time":"2026-08-19T18:01:44Z","timestamp":1787162504000},"page":"4910-4921","source":"Crossref","is-referenced-by-count":0,"title":["Go-and-Stop Nanovehicles\nEnabled by Counterbalanced\nNIR Optical Engines"],"prefix":"10.1021","volume":"6","author":[{"given":"Jing","family":"Wang","sequence":"first","affiliation":[{"name":"Shanghai University , , ,","place":["Shanghai, China, 200444"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingjing","family":"Li","sequence":"additional","affiliation":[{"name":"Shanghai University , , ,","place":["Shanghai, China, 200444"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ming","family":"Tang","sequence":"additional","affiliation":[{"name":"Chongqing General Hospital of Chongqing University & Chongqing Academy of Medical Sciences , , ,","place":["Chongqing, China, 401147"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haomin","family":"Chen","sequence":"additional","affiliation":[{"name":"Shanghai University , , ,","place":["Shanghai, China, 200444"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yaxin","family":"Sun","sequence":"additional","affiliation":[{"name":"Shanghai University , , ,","place":["Shanghai, China, 200444"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7946-8957","authenticated-orcid":true,"given":"Wenqian","family":"Chen","sequence":"additional","affiliation":[{"name":"Shanghai University , , ,","place":["Shanghai, China, 200444"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1303-0458","authenticated-orcid":true,"given":"Yong","family":"Zhang","sequence":"additional","affiliation":[{"name":"City University of Hong Kong , , SAR ,","place":["Hong Kong, China, 999077"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2815-5197","authenticated-orcid":true,"given":"Xiaohui","family":"Zhu","sequence":"additional","affiliation":[{"name":"Shanghai University , , ,","place":["Shanghai, China, 200444"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,8,19]]},"reference":[{"key":"2026092808083361200_cit1","doi-asserted-by":"publisher","first-page":"6957","DOI":"10.1002\/anie.201701396","article-title":"Magnetocatalytic Graphene\nQuantum Dots Janus Micromotors for Bacterial Endotoxin Detection","volume":"56","author":"Jurado-Sa\u0301nchez","year":"2017","journal-title":"Angew. 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