{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,22]],"date-time":"2026-09-22T14:04:02Z","timestamp":1790085842962,"version":"4.0.1"},"reference-count":44,"publisher":"American Chemical Society (ACS)","issue":"9","license":[{"start":{"date-parts":[[2026,6,11]],"date-time":"2026-06-11T00:00:00Z","timestamp":1781136000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by-nc-nd\/4.0\/"}],"funder":[{"DOI":"10.13039\/100018921","name":"Yulin Science and Technology Bureau","doi-asserted-by":"publisher","award":["2023-CXY-186"],"award-info":[{"award-number":["2023-CXY-186"]}],"id":[{"id":"10.13039\/100018921","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100021171","name":"Basic and Applied Basic Research Foundation of Guangdong Province","doi-asserted-by":"publisher","award":["2025A1515011552"],"award-info":[{"award-number":["2025A1515011552"]}],"id":[{"id":"10.13039\/501100021171","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100017596","name":"Natural Science Basic Research Program of Shaanxi Province","doi-asserted-by":"publisher","award":["2025JC-YBMS-140"],"award-info":[{"award-number":["2025JC-YBMS-140"]}],"id":[{"id":"10.13039\/501100017596","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22575192"],"award-info":[{"award-number":["22575192"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"name":"Key Research and Development Program of Xianyang City in Shaanxi Province of China","award":["L2025-ZDYF-XCL-003"],"award-info":[{"award-number":["L2025-ZDYF-XCL-003"]}]},{"name":"Qin Chuang Yuan Scientist and Engineer Team Construction Project in Shaanxi Province of China","award":["2024QCY-KXJ-121"],"award-info":[{"award-number":["2024QCY-KXJ-121"]}]},{"name":"Natural Science Foundation of Xi?an City in Shaanxi Province of China","award":["26ZRKX00007"],"award-info":[{"award-number":["26ZRKX00007"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,22]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>Wholly aromatic polyimides (PIs) are promising candidates for next-generation optoelectronic materials owing to their excellent comprehensive properties. However, the strong charge-transfer (CT) interactions present in both solution and solid states typically result in poor photoluminescence (PL) efficiency, posing a significant limitation for conventional wholly aromatic PIs for optoelectronic applications. Tetraphenylethylene (TPE), a well-established fluorophore, is well known for its straightforward synthesis, versatile functionalization capability, and high fluorescence quantum yield (\u03a6PL) even when decorated with various substituents. Thus, incorporating TPE fluorophore into the PI backbone presents a promising strategy to develop photoluminescent PIs and overcome the inherent drawbacks of traditional conjugated polymers. Herein, TPE-diamines with trans- and cis-configurations were synthesized and subsequently polymerized with 6FDA or BPADA dianhydrides to introduce TPE into the PI main chains (MC-TPE-PIs). However, the resulting MC-TPE-PIs exhibited negligible \u03a6PL, failing to deliver the anticipated emission properties. To address this limitation, a carboxyl-functionalized TPE derivative (TPE-COOH) was prepared and grafted as a side-chain substituent onto the PI backbone via esterification (SC-TPE-PIs). By tuning the flexibility and electronic effects of the dianhydrides, a series of SC-TPE-PI thin films with varying TPE contents were obtained. Among them, the highest \u03a6PL reached 13.7%, with a tensile strength of 83.3 MPa, a tensile modulus of 1.78 GPa, a glass transition temperature of 203.1 \u00b0C, and a thermal decomposition temperature of 377 \u00b0C at 5% weight loss, demonstrating their potential as luminescent polymers for optoelectronic applications.<\/jats:p>","DOI":"10.1021\/polymscitech.6c00025","type":"journal-article","created":{"date-parts":[[2026,6,11]],"date-time":"2026-06-11T12:13:23Z","timestamp":1781180003000},"page":"681-692","source":"Crossref","is-referenced-by-count":0,"title":["Tetraphenylethylene-Based\nWholly Aromatic Polyimides\nwith Enhanced Photoluminescence Efficiency"],"prefix":"10.1021","volume":"2","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-4457-2257","authenticated-orcid":true,"given":"Xingfeng","family":"Lei","sequence":"first","affiliation":[{"name":"Shenzhen Research Institute of Northwestern Polytechnical University , Sanhang Science & Technology Building, No. 45th, Gaoxin South 9th Road , Nanshan District, ,","place":["Shenzhen City, P. R. China, 518057"]},{"name":"Northwestern Polytechnical University , , , ,","place":["Xi\u2019an, Shaanxi, P. R. China, 710072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tianhao","family":"Huang","sequence":"additional","affiliation":[{"name":"Shenzhen Research Institute of Northwestern Polytechnical University , Sanhang Science & Technology Building, No. 45th, Gaoxin South 9th Road , Nanshan District, ,","place":["Shenzhen City, P. R. China, 518057"]},{"name":"Northwestern Polytechnical University , , , ,","place":["Xi\u2019an, Shaanxi, P. R. China, 710072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Liu","sequence":"additional","affiliation":[{"name":"Shenzhen Research Institute of Northwestern Polytechnical University , Sanhang Science & Technology Building, No. 45th, Gaoxin South 9th Road , Nanshan District, ,","place":["Shenzhen City, P. R. China, 518057"]},{"name":"Northwestern Polytechnical University , , , ,","place":["Xi\u2019an, Shaanxi, P. R. China, 710072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qinyu","family":"Yu","sequence":"additional","affiliation":[{"name":"Shenzhen Research Institute of Northwestern Polytechnical University , Sanhang Science & Technology Building, No. 45th, Gaoxin South 9th Road , Nanshan District, ,","place":["Shenzhen City, P. R. China, 518057"]},{"name":"Northwestern Polytechnical University , , , ,","place":["Xi\u2019an, Shaanxi, P. R. China, 710072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huajie","family":"Min","sequence":"additional","affiliation":[{"name":"Shenzhen Research Institute of Northwestern Polytechnical University , Sanhang Science & Technology Building, No. 45th, Gaoxin South 9th Road , Nanshan District, ,","place":["Shenzhen City, P. R. China, 518057"]},{"name":"Northwestern Polytechnical University , , , ,","place":["Xi\u2019an, Shaanxi, P. R. China, 710072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9377-9049","authenticated-orcid":true,"given":"Cheng","family":"Li","sequence":"additional","affiliation":[{"name":"Sun Yat-sen University , , , ,","place":["Zhuhai, Guangdong, P. R. China, 519082"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4823-5031","authenticated-orcid":true,"given":"Qiuyu","family":"Zhang","sequence":"additional","affiliation":[{"name":"Northwestern Polytechnical University , , , ,","place":["Xi\u2019an, Shaanxi, P. R. China, 710072"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5786-5660","authenticated-orcid":true,"given":"Zhaohui","family":"Wang","sequence":"additional","affiliation":[{"name":"Tsinghua University , , ,","place":["Beijing, P. R. China, 100084"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"316","published-online":{"date-parts":[[2026,6,11]]},"reference":[{"issue":"7","key":"2026092209075660200_cit1","doi-asserted-by":"publisher","first-page":"907","DOI":"10.1016\/j.progpolymsci.2012.02.005","article-title":"Advanced Polyimide\nMaterials: Syntheses, Physical Properties and\nApplications","volume":"37","author":"Liaw","year":"2012","journal-title":"Prog. Polym. Sci."},{"issue":"3","key":"2026092209075660200_cit2","doi-asserted-by":"publisher","first-page":"2101949","DOI":"10.1002\/adom.202101949","article-title":"Triarylamine-Based\nWholly Aromatic Polyimide with Simultaneously\nUnprecedented Photoluminescence Efficiency and High Glass-Transition\nTemperature","volume":"10","author":"Shao","year":"2022","journal-title":"Adv. Opt. Mater."},{"issue":"9","key":"2026092209075660200_cit3","doi-asserted-by":"publisher","first-page":"668","DOI":"10.1002\/adom.201300181","article-title":"High-Efficiency\nPhotoluminescence Wholly Aromatic Triarylamine-based Polyimide Nanofiber\nwith Aggregation-Induced Emission Enhancement","volume":"1","author":"Yen","year":"2013","journal-title":"Adv. Opt. Mater."},{"issue":"2","key":"2026092209075660200_cit4","doi-asserted-by":"publisher","first-page":"492","DOI":"10.1021\/am201509n","article-title":"Atomic Oxygen Effects on POSS Polyimides\nin Low Earth Orbit","volume":"4","author":"Minton","year":"2012","journal-title":"ACS Appl. Mater. 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C"},{"issue":"6","key":"2026092209075660200_cit17","doi-asserted-by":"publisher","first-page":"1212","DOI":"10.1021\/cm3003172","article-title":"High-Performance Functional Polyimides Containing Rigid\nNonplanar Conjugated Triphenylethylene Moieties","volume":"24","author":"Liu","year":"2012","journal-title":"Chem. Mater."},{"issue":"6","key":"2026092209075660200_cit18","doi-asserted-by":"publisher","first-page":"1302","DOI":"10.1002\/pola.26498","article-title":"Synthesis and Properties\nof High-Performance Functional Polyimides Containing Rigid Nonplanar\nConjugated Tetraphenylethylene Moieties","volume":"51","author":"Liu","year":"2013","journal-title":"J.\nPolym. Sci., Part A: Polym. Chem."},{"issue":"46","key":"2026092209075660200_cit19","doi-asserted-by":"publisher","first-page":"15212","DOI":"10.1021\/jp9072922","article-title":"Molecular\nDesign, Synthesis, and Properties of Highly Fluorescent Polyimides","volume":"113","author":"Wakita","year":"2009","journal-title":"J. Phys. Chem. B"},{"issue":"10","key":"2026092209075660200_cit20","doi-asserted-by":"publisher","first-page":"2210","DOI":"10.1002\/pola.24652","article-title":"New Polyimides Incorporated\nwith Diphenylpyrenylamine Unit as Fluorophore and Redox-Chromophore","volume":"49","author":"Kung","year":"2011","journal-title":"J. Polym. Sci., Part A: Polym. Chem."},{"issue":"6","key":"2026092209075660200_cit21","doi-asserted-by":"publisher","first-page":"630","DOI":"10.1039\/C2CC37857D","article-title":"Novel High-Efficiency\nPL Polyimide\nNanofiber Containing Aggregation-Induced Emission (AIE)-Active Cyanotriphenylamine\nLuminogen","volume":"49","author":"Yen","year":"2013","journal-title":"Chem. Commun."},{"issue":"8","key":"2026092209075660200_cit22","doi-asserted-by":"publisher","first-page":"1569","DOI":"10.1039\/C5PY01939G","article-title":"Triphenylamine-Based\nLuminogens and\nFluorescent Polyimides: Effects of Functional Groups and Substituents\non Photophysical Behaviors","volume":"7","author":"Wu","year":"2016","journal-title":"Polym. Chem."},{"issue":"15","key":"2026092209075660200_cit23","doi-asserted-by":"publisher","first-page":"4777","DOI":"10.1021\/ma971399n","article-title":"Synthesis\nand Characterization of\nA New Blue-Light-Emitting Polyimide","volume":"31","author":"Pyo","year":"1998","journal-title":"Macromolecules"},{"issue":"1","key":"2026092209075660200_cit24","doi-asserted-by":"publisher","first-page":"125","DOI":"10.1016\/S0032-3861(98)00231-6","article-title":"Synthesis and Blue Light-Emitting\nCharacteristic of\nRod-Like Poly(4,4\u2032-biphenylene pyromellitimide) with Furyl\nSide Groups","volume":"40","author":"Pyo","year":"1999","journal-title":"Polymer"},{"issue":"32","key":"2026092209075660200_cit25","doi-asserted-by":"publisher","first-page":"4985","DOI":"10.1039\/D2CC00722C","article-title":"Effect of Solvation\non the Aggregation-Induced Luminescence of Tetraphenylethene Derivatives","volume":"58","author":"Yao","year":"2022","journal-title":"Chem. Commun."},{"issue":"40","key":"2026092209075660200_cit26","doi-asserted-by":"publisher","first-page":"12709","DOI":"10.1039\/C9TC04501E","article-title":"The Influence of Intermolecular Interactions\nand Molecular\nPackings on Mechanochromism and Mechanoluminescence-A Tetraphenylethylene\nDerivative Case","volume":"7","author":"Huang","year":"2019","journal-title":"J. Mater. Chem. C"},{"issue":"6","key":"2026092209075660200_cit27","doi-asserted-by":"publisher","first-page":"1037","DOI":"10.1039\/C6CC09106G","article-title":"Dual Aggregation-Induced\nEmission for Enhanced Fluorescence Sensing\nof Furin Activity in Vitro and in Living Cells","volume":"53","author":"Liu","year":"2017","journal-title":"Chem. Commun."},{"issue":"5","key":"2026092209075660200_cit28","doi-asserted-by":"publisher","first-page":"2290","DOI":"10.1021\/acsapm.1c00182","article-title":"Photoresponsive\nPolymers with Aggregation-Induced Emission","volume":"3","author":"Du","year":"2021","journal-title":"ACS Appl. Polym. Mater."},{"issue":"4","key":"2026092209075660200_cit29","doi-asserted-by":"publisher","first-page":"289","DOI":"10.1007\/s10118-019-2221-4","article-title":"Recent\nProgress in AIE-active Polymers","volume":"37","author":"Hu","year":"2019","journal-title":"Chin. J. Polym.\nSci."},{"issue":"13","key":"2026092209075660200_cit30","doi-asserted-by":"publisher","first-page":"2572","DOI":"10.1021\/acs.jpca.7b00197","article-title":"Excited-State Decay Paths in Tetraphenylethene Derivatives","volume":"121","author":"Gao","year":"2017","journal-title":"J. Phys. Chem. A"},{"issue":"12","key":"2026092209075660200_cit31","doi-asserted-by":"publisher","first-page":"4932","DOI":"10.1021\/acs.macromol.0c00311","article-title":"Catalyst-Free Click Polymerization\nof Thiol and Activated Internal\nAlkynes: A Facile Strategy toward Functional Poly(\u03b2-thioacrylate)s","volume":"53","author":"Du","year":"2020","journal-title":"Macromolecules"},{"issue":"1","key":"2026092209075660200_cit32","doi-asserted-by":"publisher","first-page":"1","DOI":"10.1007\/s40242-021-0381-6","article-title":"Restriction of Intramolecular\nMotion(RIM): Investigating AIE Mechanism from Experimental and Theoretical\nStudies","volume":"37","author":"Zhang","year":"2021","journal-title":"Chem. Res. Chin. Univ."},{"issue":"1","key":"2026092209075660200_cit33","doi-asserted-by":"publisher","first-page":"011111","DOI":"10.1063\/1.2753723","article-title":"Aggregation-Induced\nEmissions of Tetraphenylethene Derivatives and Their Utilities as\nChemical Vapor Sensors and in Organic Light-Emitting Diodes","volume":"91","author":"Dong","year":"2007","journal-title":"Appl. Phys. Lett."},{"issue":"38","key":"2026092209075660200_cit34","doi-asserted-by":"publisher","first-page":"11790","DOI":"10.1039\/C9TC04140K","article-title":"Insight from the Old: Mechanochromism\nand Mechanoluminescence\nof Two Amine-Containing Tetraphenylethylene Isomers","volume":"7","author":"Jiang","year":"2019","journal-title":"J. Mater. Chem. C"},{"issue":"44","key":"2026092209075660200_cit35","doi-asserted-by":"publisher","first-page":"5598","DOI":"10.1039\/C8CC03083A","article-title":"Opposite Mechanoluminescence\nBehavior of Two Isomers with Different\nLinkage Positions","volume":"54","author":"Liu","year":"2018","journal-title":"Chem. Commun."},{"issue":"2","key":"2026092209075660200_cit36","doi-asserted-by":"publisher","first-page":"885","DOI":"10.1039\/D0QM00720J","article-title":"Cyano-Containing\nTetraphenylethene Isomers: Similar Bright Mechanoluminescence, but\nDiverse Recoverable Processes","volume":"5","author":"Jiang","year":"2021","journal-title":"Mater. Chem.\nFront."},{"issue":"30","key":"2026092209075660200_cit37","doi-asserted-by":"publisher","first-page":"34198","DOI":"10.1021\/acsami.0c08480","article-title":"Preserving High-Efficiency\nLuminescence Characteristics of an Aggregation-Induced Emission-Active\nFluorophore in Thermostable Amorphous Polymers","volume":"12","author":"Zhou","year":"2020","journal-title":"ACS Appl. Mater. Interfaces"},{"issue":"1","key":"2026092209075660200_cit38","doi-asserted-by":"publisher","first-page":"331","DOI":"10.1002\/anie.202013183","article-title":"Diels-Alder\nPolymer Networks with Temperature-Reversible\nCross-Linking-Induced Emission","volume":"60","author":"Jiang","year":"2021","journal-title":"Angew. Chem.,\nInt. Ed."},{"key":"2026092209075660200_cit39","doi-asserted-by":"publisher","first-page":"125579","DOI":"10.1016\/j.polymer.2022.125579","article-title":"Colorless Polyimide Films with Low\nBirefringence and Retardation: Synthesis and Characterization","volume":"265","author":"Li","year":"2023","journal-title":"Polymer"},{"key":"2026092209075660200_cit40","doi-asserted-by":"publisher","first-page":"83","DOI":"10.1016\/j.polymer.2016.01.037","article-title":"Conformational Characterization of Imide Compounds and Polyimides\nUsing Far-Infrared Spectroscopy and DFT Calculations","volume":"86","author":"Okada","year":"2016","journal-title":"Polymer"},{"issue":"18","key":"2026092209075660200_cit41","doi-asserted-by":"publisher","first-page":"1740","DOI":"10.1039\/b105159h","article-title":"Aggregation-Induced Emission of 1-Methyl-1,2,3,4,5-Pentaphenylsilole","author":"Luo","year":"2001","journal-title":"Chem. Commun."},{"issue":"21","key":"2026092209075660200_cit42","doi-asserted-by":"publisher","first-page":"11718","DOI":"10.1021\/acs.chemrev.5b00263","article-title":"Aggregation-Induced\nEmission: Together We Shine, United We Soar!","volume":"115","author":"Mei","year":"2015","journal-title":"Chem. Rev."},{"issue":"11","key":"2026092209075660200_cit43","doi-asserted-by":"publisher","first-page":"5361","DOI":"10.1039\/c1cs15113d","article-title":"Aggregation-Induced\nEmission","volume":"40","author":"Hong","year":"2011","journal-title":"Chem. Soc. Rev."},{"issue":"45","key":"2026092209075660200_cit44","doi-asserted-by":"publisher","first-page":"11874","DOI":"10.1039\/C5TC02790J","article-title":"A Thermally\nStable and Reversible Microporous Hydrogen-Bonded Organic Framework:\nAggregation Induced Emission and Metal Ion-Sensing Properties","volume":"3","author":"Zhou","year":"2015","journal-title":"J. Mater. Chem. C"}],"container-title":["Polymer Science &amp; Technology"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/polymscitech.6c00025","content-type":"application\/pdf","content-version":"vor","intended-application":"unspecified"},{"URL":"https:\/\/pubs.acs.org\/pstoco\/article-pdf\/2\/9\/681\/66265166\/polymscitech.6c00025.pdf","content-type":"application\/pdf","content-version":"vor","intended-application":"syndication"},{"URL":"https:\/\/pubs.acs.org\/pstoco\/article-pdf\/2\/9\/681\/66265166\/polymscitech.6c00025.pdf","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,9,22]],"date-time":"2026-09-22T13:31:33Z","timestamp":1790083893000},"score":1,"resource":{"primary":{"URL":"https:\/\/pubs.acs.org\/pstoco\/article\/2\/9\/681\/5233094\/Tetraphenylethylene-Based-Wholly-Aromatic"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,6,11]]},"references-count":44,"journal-issue":{"issue":"9","published-online":{"date-parts":[[2026,6,11]]},"published-print":{"date-parts":[[2026,9,22]]}},"URL":"https:\/\/doi.org\/10.1021\/polymscitech.6c00025","relation":{},"ISSN":["2997-3279"],"issn-type":[{"value":"2997-3279","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,6,11]]}}}