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Chem."},{"key":"ref45\/cit45","doi-asserted-by":"crossref","first-page":"33","DOI":"10.1016\/0263-7855(96)00018-5","volume":"14","author":"Humphrey W.","year":"1996","journal-title":"J. Mol. Graph."},{"key":"ref46\/cit46","doi-asserted-by":"crossref","first-page":"6269","DOI":"10.1021\/j100308a038","volume":"91","author":"Berendsen H. J. C.","year":"1987","journal-title":"J. Phys. Chem."},{"key":"ref47\/cit47","doi-asserted-by":"crossref","first-page":"245","DOI":"10.1016\/j.cplett.2005.10.135","volume":"418","author":"Lamoureux G.","year":"2006","journal-title":"Chem. Phys. Lett."},{"key":"ref48\/cit48","doi-asserted-by":"crossref","first-page":"842","DOI":"10.1016\/S0009-2614(03)00526-8","volume":"372","author":"Lawrence C. P.","year":"2003","journal-title":"Chem. Phys. Lett."},{"key":"ref49\/cit49","doi-asserted-by":"crossref","first-page":"2356","DOI":"10.1063\/1.470931","volume":"104","author":"Rey R.","year":"1996","journal-title":"J. Chem. 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Phys."},{"key":"ref55\/cit55","doi-asserted-by":"crossref","first-page":"8510","DOI":"10.1063\/1.480192","volume":"111","author":"Trokhymchuk A.","year":"1999","journal-title":"J. Chem. Phys."},{"key":"ref56\/cit56","doi-asserted-by":"crossref","first-page":"87","DOI":"10.1021\/jz101461d","volume":"2","author":"Jiang W.","year":"2010","journal-title":"J. Phys. Chem. Lett."},{"key":"ref57\/cit57","unstructured":"Wood, W. W.InPhysics of Simple Liquids;Temperley, H. N. V.; Rowlinson, J. S.; Rushbrooke, G. S., Eds.North-Holland publishing Co.:Amsterdam, 1968; Chapter 5, pp151\u2013155."},{"key":"ref58\/cit58","doi-asserted-by":"crossref","first-page":"5437","DOI":"10.1021\/jp9703059","volume":"101","author":"Chitra R.","year":"1997","journal-title":"J. Phys. Chem. B"},{"key":"ref59\/cit59","doi-asserted-by":"crossref","first-page":"103","DOI":"10.1081\/ASR-200038326","volume":"40","author":"Lambert A. G.","year":"2005","journal-title":"Appl. Spectrosc. Rev."},{"key":"ref60\/cit60","doi-asserted-by":"crossref","unstructured":"Heinz, T. F.InNonlinear Surface Electromagnetic Phenomena;Ponrath, H. E.; Stegeman, G. I., Eds.Elsevier Science Publishers:Amsterdam, 1991; pp353\u2013416.","DOI":"10.1016\/B978-0-444-88359-9.50011-9"},{"key":"ref61\/cit61","doi-asserted-by":"crossref","first-page":"12632","DOI":"10.1103\/PhysRevB.59.12632","volume":"59","author":"Zhuang X.","year":"1999","journal-title":"Phys. Rev. B"},{"key":"ref62\/cit62","first-page":"13","volume":"66","author":"Wei X.","year":"2002","journal-title":"Phys. Rev. B"},{"key":"ref63\/cit63","doi-asserted-by":"crossref","first-page":"2536","DOI":"10.1021\/jp200757x","volume":"115","author":"Laaser J. E.","year":"2011","journal-title":"J. Phys. Chem. B"},{"key":"ref64\/cit64","doi-asserted-by":"crossref","first-page":"192","DOI":"10.1038\/nature10173","volume":"474","author":"Stiopkin I. 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