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Horizontal mesh refinement in CESM\/CAM\u2010chem\u2010SE is unique and novel in that pollutants such as ozone are accurately represented at human exposure relevant scales while also directly including global feedbacks. CESM\/CAM\u2010chem\u2010SE with mesh refinement down to \u223c14\u00a0km over the conterminous US (CONUS) is the beginning of the Multi\u2010Scale Infrastructure for Chemistry and Aerosols (MUSICAv0). Here, MUSICAv0 is evaluated and used to better understand how horizontal resolution and chemical complexity impact ozone and ozone precursors over CONUS as compared to measurements from five aircraft campaigns, which occurred in 2013. This field campaign analysis demonstrates the importance of using finer horizontal resolution to accurately simulate ozone precursors such as nitrogen oxides and carbon monoxide. In general, the impact of using more complex chemistry on ozone and other oxidation products is more pronounced when using finer horizontal resolution where a larger number of chemical regimes are resolved. Large model biases for ozone near the surface remain in the Southeast US as compared to the aircraft observations even with updated chemistry and finer horizontal resolution. This suggests a need for adding the capability of replacing sections of global emission inventories with regional inventories, increasing the vertical resolution in the planetary boundary layer, and reducing model biases in meteorological variables such as temperature and clouds.<\/jats:p>","DOI":"10.1029\/2021ms002889","type":"journal-article","created":{"date-parts":[[2022,5,21]],"date-time":"2022-05-21T05:29:21Z","timestamp":1653110961000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":48,"title":["Evaluating the Impact of Chemical Complexity and Horizontal Resolution on Tropospheric Ozone Over the Conterminous US With a Global Variable Resolution Chemistry Model"],"prefix":"10.1029","volume":"14","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-7095-3718","authenticated-orcid":false,"given":"Rebecca H.","family":"Schwantes","sequence":"first","affiliation":[{"name":"Atmospheric Chemistry Observations &amp; Modeling Laboratory National Center for Atmospheric Research  Boulder CO USA"},{"name":"Cooperative Institute for Research in Environmental Sciences University of Colorado Boulder  Boulder CO USA"},{"name":"Chemical Sciences Laboratory National Oceanic and Atmospheric Administration  Boulder CO USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4578-8375","authenticated-orcid":false,"given":"Forrest G.","family":"Lacey","sequence":"additional","affiliation":[{"name":"Atmospheric Chemistry Observations &amp; 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