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We report the first model of stratospheric mercury chemistry based on a novel photosensitized oxidation mechanism. We find two very distinct Hg chemical regimes in the stratosphere: in the upper stratosphere, above the ozone maximum concentration, Hg\n                    <jats:sup>0<\/jats:sup>\n                    oxidation is initiated by photosensitized reactions, followed by second\u2010step chlorine chemistry. In the lower stratosphere, ground\u2010state Hg\n                    <jats:sup>0<\/jats:sup>\n                    is oxidized by thermal reactions at much slower rates. This dichotomy arises due to the coincidence of the mercury absorption at 253.7\u00a0nm with the ozone Hartley band maximum at 254\u00a0nm. We also find that stratospheric Hg oxidation, controlled by chlorine and hydroxyl radicals, is much faster than previously assumed, but moderated by efficient photo\u2010reduction of mercury compounds. Mercury lifetime shows a steep increase from hours in the upper\u2010middle stratosphere to years in the lower stratosphere.\n                  <\/jats:p>","DOI":"10.1029\/2022gl097953","type":"journal-article","created":{"date-parts":[[2022,5,31]],"date-time":"2022-05-31T13:47:07Z","timestamp":1654004827000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":20,"title":["The Chemistry of Mercury in the Stratosphere"],"prefix":"10.1029","volume":"49","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-0060-1581","authenticated-orcid":false,"given":"Alfonso","family":"Saiz\u2010Lopez","sequence":"first","affiliation":[{"name":"Department of Atmospheric Chemistry and Climate Institute of Physical Chemistry Rocasolano CSIC  Madrid Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"A. 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