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However, the application of such zeolites is limited by a rapid deactivation due to coke formation. We present a novel catalyst design concept to significantly enhance coke resistance, achieved by physically mixing the zeolite with a secondary catalyst component exhibiting hydrogenation activity and operating under near ambient-pressure hydrogen co-feeds. Among the tested materials, Pd\/SiO\n                    <jats:sub>2<\/jats:sub>\n                    provides the highest stability enhancement, leading up to 10\u00d7 higher cumulative productivity of C\n                    <jats:sub>3<\/jats:sub>\n                    \u2013C\n                    <jats:sub>5<\/jats:sub>\n                    alkenes, and outperforming a bifunctional Pd-loaded zeolite. The enhancement is observed across a broad range of hydrogen concentrations and zeolite:Pd\/SiO\n                    <jats:sub>2<\/jats:sub>\n                    weight ratios, offering flexibility to minimize hydrogen and Pd use. Kinetic and spectroscopic investigations reveal that Pd intercepts coke-forming intermediates, such as formaldehyde and dienes, thereby reducing the rate of internal and external coke deposition.\n                  <\/jats:p>","DOI":"10.1038\/s41467-026-77944-9","type":"journal-article","created":{"date-parts":[[2026,9,23]],"date-time":"2026-09-23T17:11:27Z","timestamp":1790183487000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Enhanced alkene productivity in methanol-to-hydrocarbons conversion using a secondary catalyst component and hydrogen co-feeds"],"prefix":"10.1038","volume":"17","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-3657-9638","authenticated-orcid":false,"given":"Matteo","family":"Vanni","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7863-8763","authenticated-orcid":false,"given":"Andreas","family":"Brenig","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5478-9639","authenticated-orcid":false,"given":"Adam H.","family":"Clark","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4166-2284","authenticated-orcid":false,"given":"Jeroen A.","family":"van Bokhoven","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6630-1672","authenticated-orcid":false,"given":"Vladimir","family":"Paunovi\u0107","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,9,23]]},"reference":[{"key":"77944_CR1","doi-asserted-by":"publisher","first-page":"5810","DOI":"10.1002\/anie.201103657","volume":"51","author":"U Olsbye","year":"2012","unstructured":"Olsbye, U. et al. 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