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Notably, this strategy can be directly applied to crude commercial polymers, does not rely on preinstalled end-groups or sacrificial co-monomers, operates at relatively low temperatures in the absence of light irradiation and precludes the use of a solvent, therefore enabling direct isolation of pristine monomers in high yields (\u223c90%). The methodology is compatible with polymethacrylates synthesized by either anionic, free radical or controlled radical polymerization and can also be applied to ultrahigh-molecular-weight materials (&gt;10\n                    <jats:sup>6<\/jats:sup>\n                    \u2009Da).\n                  <\/jats:p>","DOI":"10.1038\/s41557-026-02232-4","type":"journal-article","created":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T09:03:05Z","timestamp":1788339785000},"page":"1979-1987","update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Lower-temperature bulk depolymerization of commercial polymethacrylates"],"prefix":"10.1038","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-4787-2060","authenticated-orcid":false,"given":"Richard","family":"Whitfield","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5516-7439","authenticated-orcid":false,"given":"Victoria","family":"Lohmann","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mikhail","family":"Agrachev","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9469-6699","authenticated-orcid":false,"given":"Hongsik","family":"Kim","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2515-3906","authenticated-orcid":false,"given":"Hyun Suk","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nethmi","family":"De Alwis Watuthanthrige","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9900-2644","authenticated-orcid":false,"given":"Nghia P.","family":"Truong","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9521-6450","authenticated-orcid":false,"given":"Tae-Lim","family":"Choi","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6853-8585","authenticated-orcid":false,"given":"Gunnar","family":"Jeschke","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6615-1026","authenticated-orcid":false,"given":"Athina","family":"Anastasaki","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"297","published-online":{"date-parts":[[2026,9,2]]},"reference":[{"key":"2232_CR1","doi-asserted-by":"crossref","first-page":"496","DOI":"10.3390\/nano11020496","volume":"11","author":"MS-L Yee","year":"2021","unstructured":"Yee, M. 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