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materials is an emerging field in materials science, with important applications on alternative solid-state cooling technologies, energy harvesting and sensors\/actuators. In this direction, we developed a thorough investigation of a multiferroic composite, comprising magnetocaloric\/magnetostrictive Gd<jats:inline-formula><jats:alternatives><jats:tex-math>$${}_{5}$$<\/jats:tex-math><mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\">\n                  <mml:msub>\n                    <mml:mrow\/>\n                    <mml:mrow>\n                      <mml:mn>5<\/mml:mn>\n                    <\/mml:mrow>\n                  <\/mml:msub>\n                <\/mml:math><\/jats:alternatives><\/jats:inline-formula>Si<jats:inline-formula><jats:alternatives><jats:tex-math>$${}_{2.4}$$<\/jats:tex-math><mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\">\n                  <mml:msub>\n                    <mml:mrow\/>\n                    <mml:mrow>\n                      <mml:mn>2.4<\/mml:mn>\n                    <\/mml:mrow>\n                  <\/mml:msub>\n                <\/mml:math><\/jats:alternatives><\/jats:inline-formula>Ge<jats:inline-formula><jats:alternatives><jats:tex-math>$${}_{1.6}$$<\/jats:tex-math><mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\">\n                  <mml:msub>\n                    <mml:mrow\/>\n                    <mml:mrow>\n                      <mml:mn>1.6<\/mml:mn>\n                    <\/mml:mrow>\n                  <\/mml:msub>\n                <\/mml:math><\/jats:alternatives><\/jats:inline-formula> microparticles blended into a piezo- and pyroelectric poly(vinylidene) fluoride (PVDF) matrix. Using a simple solvent casting technique, the formation and stabilization of PVDF electroactive phases are improved when the filler content increases from 2 to 12 weight fraction (wt.%). This effect greatly contributes to the magnetoelectric (ME) coupling, with the ME coefficient <jats:inline-formula><jats:alternatives><jats:tex-math>$${\\alpha }_{ME}$$<\/jats:tex-math><mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\">\n                  <mml:msub>\n                    <mml:mrow>\n                      <mml:mi>\u03b1<\/mml:mi>\n                    <\/mml:mrow>\n                    <mml:mrow>\n                      <mml:mi>M<\/mml:mi>\n                      <mml:mi>E<\/mml:mi>\n                    <\/mml:mrow>\n                  <\/mml:msub>\n                <\/mml:math><\/jats:alternatives><\/jats:inline-formula> increasing from 0.3 V\/cm.Oe to 2.2 V\/cm.Oe, by increasing the amount of magnetic material. In addition, magnetic measurements revealed that the ME-coupling has influenced the magnetocaloric effect via a contribution from the electroactive polymer and hence leading to a multicaloric effect. These results contribute to the development of multifunctional systems for novel technologies.<\/jats:p>","DOI":"10.1038\/s41598-019-54635-8","type":"journal-article","created":{"date-parts":[[2019,12,4]],"date-time":"2019-12-04T11:02:34Z","timestamp":1575457354000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":28,"title":["Multicaloric effect in a multiferroic composite of Gd5(Si,Ge)4 microparticles embedded into a ferroelectric PVDF matrix"],"prefix":"10.1038","volume":"9","author":[{"given":"V. 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