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An approximate Gaussian distribution of nanospheres with a mean diameter of 4.5 nm and a standard deviation of 1.1 nm, as determined by atomic force microscopy, is provided by the intrinsic granularity of an ultrathin, gold film, having a nominal thickness of \u22480.18 nm. The cavity ring-down measurements employ a linear resonator with an intracavity flow cell, which is formed by a pair of ultrasmooth, fused-silica optical flats at Brewster\u2019s angle, where the Au film is present on a single flat. The total system intrinsic loss is dominated by the film extinction, while the angled flats alone contribute only \u22485\u00d710\u22125\/flat to the total loss. Based on a relative ring-down time precision of 0.1% for ensembles averages of 25 laser shots from a pulsed optical parametric oscillator, the minimum detectable concentrations of PCE and TCE obtained by probing the SPR response are found to be 2 and 7\u00d710\u22128\u2009mol\/L, respectively, based on a 30 s integration time.<\/jats:p>","DOI":"10.1063\/1.1629279","type":"journal-article","created":{"date-parts":[[2004,1,9]],"date-time":"2004-01-09T23:10:48Z","timestamp":1073689848000},"page":"1585-1593","update-policy":"http:\/\/dx.doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":23,"title":["Surface-plasmon-resonance-enhanced cavity ring-down detection"],"prefix":"10.1063","volume":"120","author":[{"given":"Andrew C. 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