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Zn deposition at LT, at 105\u00a0K (STM) or 80\u00a0K (XPS), leads to nucleation and two-dimensional growth of Zn islands mainly at the elbows of the Au(111) herringbone reconstruction, with a slight preference for island formation at pinched-in (pi) rather than bulged-out (bu) elbows. Local surface intermixing during LT Zn deposition leads to local perturbations of the Au(111) herringbone reconstruction, which results in the formation of additional nucleation sites (edge sites). At higher coverages (&amp;gt;0.11 ML), island coalescence sets in. Testing the thermal stability by annealing experiments, we find the structures to be stable up to about 200\u00a0K, while at higher temperatures, 2D sintering, intermixing, and dissolution set in, with subtle differences between pi- and bu-elbow islands. This indicates largely comparable activation barriers for the underlying (surface-)diffusion and exchange processes. Upon annealing to 330\u00a0K, all island structures dissolved. Compared with previous reports on the growth of other metals on Au(111), Zn shows a rather high tendency for intermixing and can be considered to be typical of metal deposition systems with comparable barriers for 2D Zn detachment\/sintering and intermixing\/bulk diffusion.<\/jats:p>","DOI":"10.1063\/5.0054980","type":"journal-article","created":{"date-parts":[[2021,9,30]],"date-time":"2021-09-30T09:52:23Z","timestamp":1632995543000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":2,"title":["Low-temperature nucleation and growth of Zn on Au(111) and thermal stability toward (surface) alloy formation"],"prefix":"10.1063","volume":"155","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3827-5555","authenticated-orcid":false,"given":"Konstantin M.","family":"Sch\u00fcttler","sequence":"first","affiliation":[{"name":"Institute of Surface Chemistry and Catalysis, Ulm University , Albert-Einstein-Allee 47, D-89081 Ulm, Germany"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3205-7450","authenticated-orcid":false,"given":"Joachim","family":"Bansmann","sequence":"additional","affiliation":[{"name":"Institute of Surface Chemistry and Catalysis, Ulm University , Albert-Einstein-Allee 47, D-89081 Ulm, Germany"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9686-3948","authenticated-orcid":false,"given":"Albert K.","family":"Engstfeld","sequence":"additional","affiliation":[{"name":"Institute of Surface Chemistry and Catalysis, Ulm University , Albert-Einstein-Allee 47, D-89081 Ulm, Germany"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7565-0628","authenticated-orcid":false,"given":"R. 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