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Here, we computationally examine the beginnings of exciton condensation in a double layer composed of coronene, a seven-benzene-ring patch of graphene. As a function of interlayer separation, we compute the exciton population in a single coherent quantum state, showing that the population peaks around 1.8 at distances near 2 \u00c5. Visualization reveals interlayer excitons at the separation distance of the condensate. We determine the exciton population as a function of the twist angle between two coronene layers to reveal the magic angles at which the condensation peaks. As with previous recent calculations showing some exciton condensation in hexacene double layers and benzene stacks, the present two-electron reduced-density-matrix calculations with coronene provide computational evidence for the ability to realize exciton condensation in molecular-scale analogs of extended systems such as the graphene double layer.<\/jats:p>","DOI":"10.1063\/5.0084564","type":"journal-article","created":{"date-parts":[[2022,4,18]],"date-time":"2022-04-18T14:24:35Z","timestamp":1650291875000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":12,"title":["Beginnings of exciton condensation in coronene analog of graphene double layer"],"prefix":"10.1063","volume":"156","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-6760-9134","authenticated-orcid":false,"given":"LeeAnn M.","family":"Sager","sequence":"first","affiliation":[{"name":"Department of Chemistry and The James Franck Institute, The University of Chicago , Chicago, Illinois 60637, USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6425-5219","authenticated-orcid":false,"given":"Anna O.","family":"Schouten","sequence":"additional","affiliation":[{"name":"Department of Chemistry and The James Franck Institute, The University of Chicago , Chicago, Illinois 60637, USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9938-3886","authenticated-orcid":false,"given":"David A.","family":"Mazziotti","sequence":"additional","affiliation":[{"name":"Department of Chemistry and The James Franck Institute, The University of Chicago , Chicago, Illinois 60637, USA"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"317","published-online":{"date-parts":[[2022,4,18]]},"reference":[{"key":"2023081004534907900_c1","doi-asserted-by":"publisher","first-page":"036801","DOI":"10.1103\/PhysRevLett.93.036801","article-title":"Vanishing Hall resistance at high magnetic field in a double-layer two-dimensional electron system","volume":"93","year":"2004","journal-title":"Phys. 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