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Anomalous enhanced stimulated Raman scattering (SRS) of cyclohexane\u2013benzene mixtures was obtained in this study. SRS of the pure solvent, the multi-order Stokes of the strongest fundamental vibration modes, and energy transfer in intra-molecular modes were observed. SRS of the mixture revealed that the cross-pumping effect was generated between the C\u2013H stretching (v2) mode of cyclohexane and the C=C ring skeleton (v1) mode of benzene, thereby producing the intermolecular secondary stimulated Raman emission and the appearance of two super-broadband radiations at 664.36\u2013673.9\u00a0nm and 704.62\u2013729.22\u00a0nm. The results suggest that the energy transfer of intermolecular vibrational modes, where the strongest vibrational mode excites other vibrational modes, is a simple approach for generating supercontinuum coherent radiation.<\/jats:p>","DOI":"10.1063\/5.0137238","type":"journal-article","created":{"date-parts":[[2023,1,23]],"date-time":"2023-01-23T16:04:48Z","timestamp":1674489888000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":4,"title":["Intermolecular energy transfer-enhanced super-broadband stimulated Raman scattering in cyclohexane\u2013benzene mixtures"],"prefix":"10.1063","volume":"158","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-3509-0910","authenticated-orcid":false,"given":"Panpan","family":"Ren","sequence":"first","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chong","family":"Wang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bo","family":"Yang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lu","family":"Xing","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9586-2997","authenticated-orcid":false,"given":"Shenghan","family":"Wang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1904-7461","authenticated-orcid":false,"given":"Zhiwei","family":"Men","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chenglin","family":"Sun","sequence":"additional","affiliation":[{"name":"Key Laboratory of Physics and Technology for Advanced Batteries, College of Physics, Jilin University 1 , Changchun 130012, China"},{"name":"College of Physics, Jilin University 2 , Changchun 130012, China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"317","published-online":{"date-parts":[[2023,2,8]]},"reference":[{"key":"2023081022181312400_c1","doi-asserted-by":"publisher","first-page":"201","DOI":"10.1016\/s0079-6638(08)00204-7","volume":"53","year":"2009","journal-title":"Prog. 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