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Combining experimental NIPE spectra and theoretical calculations, various Gly\u00b7X\u2212 complexes were found to adopt the same types of low-lying isomers, albeit with different relative energies. Despite more congested spectral profiles for Gly\u00b7Cl\u2212 and Gly\u00b7Br\u2212, spectral assignments were accomplished with the guidance of the knowledge learned from Gly\u00b7I\u2212, where a larger spin\u2013orbit splitting of iodine afforded well-resolved, recognizable spectral peaks. Three canonical plus one zwitterionic isomer for Gly\u00b7Cl\u2212 and four canonical conformers for Gly\u00b7Br\u2212 were experimentally identified and characterized in contrast to the five canonical ones observed for Gly\u00b7I\u2212 under similar experimental conditions. Taken together, this study investigates both genericity and variations in binding patterns for the complexes composed of glycine and various halides, demonstrating that iodide-tagging is an effective spectroscopic means to unravel diverse ion-molecule binding motifs for cluster anions with congested spectral bands by substituting the respective ion with iodide.<\/jats:p>","DOI":"10.1063\/5.0159326","type":"journal-article","created":{"date-parts":[[2023,7,19]],"date-time":"2023-07-19T18:10:31Z","timestamp":1689790231000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":3,"title":["How generic is iodide-tagging photoelectron spectroscopy: An extended investigation on the Gly\u00b7<i>X<\/i>\u2212 (Gly = glycine, <i>X<\/i> = Cl or Br) complexes"],"prefix":"10.1063","volume":"159","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-2852-4047","authenticated-orcid":false,"given":"Wenjin","family":"Cao","sequence":"first","affiliation":[{"name":"Physical Sciences Division, Pacific Northwest National Laboratory 1 , Richland, Washington 99352, USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Qinqin","family":"Yuan","sequence":"additional","affiliation":[{"name":"Physical Sciences Division, Pacific Northwest National Laboratory 1 , Richland, Washington 99352, USA"},{"name":"Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Ministry of Education), Department of Chemistry, Anhui University 2 , Hefei 230601, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9011-3716","authenticated-orcid":false,"given":"Hanhui","family":"Zhang","sequence":"additional","affiliation":[{"name":"Physical Sciences Division, Pacific Northwest National Laboratory 1 , Richland, Washington 99352, USA"},{"name":"Hefei National Laboratory for Physical Sciences at the Microscale, Department of Chemical Physics, University of Science and Technology of China 3 , Hefei, Anhui 230026, People\u2019s Republic of China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0264-0146","authenticated-orcid":false,"given":"Xiaoguo","family":"Zhou","sequence":"additional","affiliation":[{"name":"Hefei National Laboratory for Physical Sciences at the Microscale, Department of Chemical Physics, University of Science and Technology of China 3 , Hefei, Anhui 230026, People\u2019s Republic of China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7007-9322","authenticated-orcid":false,"given":"Steven R.","family":"Kass","sequence":"additional","affiliation":[{"name":"Department of Chemistry, University of Minnesota 4 , Minneapolis, Minnesota 55455, USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8326-1780","authenticated-orcid":false,"given":"Xue-Bin","family":"Wang","sequence":"additional","affiliation":[{"name":"Physical Sciences Division, Pacific Northwest National Laboratory 1 , Richland, Washington 99352, USA"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"317","published-online":{"date-parts":[[2023,7,19]]},"reference":[{"key":"2023083017351184300_c1","doi-asserted-by":"publisher","first-page":"4226","DOI":"10.1021\/ja00351a017","article-title":"Effect of solvation on the acid\/base properties of glycine","volume":"105","year":"1983","journal-title":"J. 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