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In this work, we investigate the chemiresistive effect of the p-type delafossite CuScO2 microsheets by comparing their responses to various gaseous alcohols, which increase with an approximately linear relationship with the length of straight carbon chains from methanol to n-hexanol. A new mechanism is proposed to elucidate such a dramatic trend of observed chemiresistive change based on the first-principles calculations and test results. The increasing carbon chain length modulates the adsorption configuration and provides supplementary routes for electron transfer, which is assumed to account for the observed chemiresistive effect. This work may provide a novel perspective for the investigation and development of more advanced functional oxides for electrical applications.<\/jats:p>","DOI":"10.1063\/5.0206331","type":"journal-article","created":{"date-parts":[[2024,8,2]],"date-time":"2024-08-02T12:15:13Z","timestamp":1722600913000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":2,"title":["Chemiresistive effect of p-type delafossite CuScO2 microsheets to gaseous alcohols"],"prefix":"10.1063","volume":"161","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-2616-7437","authenticated-orcid":false,"given":"Hai","family":"Liu","sequence":"first","affiliation":[{"name":"Key Laboratory of Advanced Display and System Applications of Ministry of Education, Shanghai University 1 , 149 Yanchang Road, Shanghai 200072, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-8418-8975","authenticated-orcid":false,"given":"Yu","family":"Zong","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Display and System Applications of Ministry of Education, Shanghai University 1 , 149 Yanchang Road, Shanghai 200072, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Tingting","family":"Zhao","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Display and System Applications of Ministry of Education, Shanghai University 1 , 149 Yanchang Road, Shanghai 200072, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0871-5882","authenticated-orcid":false,"given":"Zhi","family":"Yang","sequence":"additional","affiliation":[{"name":"Department of Micro\/Nano Electronics, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University 2 , Shanghai 200240, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Lunchao","family":"Zhong","sequence":"additional","affiliation":[{"name":"State Key Laboratory of NBC Protection for Civilian 3 , Beijing 102205, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1121-0508","authenticated-orcid":false,"given":"Wenhuan","family":"Zhu","sequence":"additional","affiliation":[{"name":"Department of Micro\/Nano Electronics, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University 2 , Shanghai 200240, China"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"317","published-online":{"date-parts":[[2024,8,2]]},"reference":[{"key":"2024080212104471800_c1","first-page":"521","article-title":"Sensing materials: Nanofibers produced by electrospinning and solution blow spinning","volume-title":"Encyclopedia of Sensors and Biosensors","author":"Narayan","year":"2023","edition":"1"},{"issue":"1","key":"2024080212104471800_c2","doi-asserted-by":"publisher","first-page":"153","DOI":"10.1021\/nn101995f","article-title":"On the sensing mechanism in carbon nanotube chemiresistors","volume":"5","year":"2011","journal-title":"ACS Nano"},{"key":"2024080212104471800_c3","doi-asserted-by":"publisher","first-page":"1163","DOI":"10.1016\/j.snb.2017.07.146","article-title":"Effect of palladium nanoparticle functionalization on the hydrogen gas sensing of graphene based chemi-resistive devices","volume":"253","year":"2017","journal-title":"Sens. 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