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These states were formed using circularly or elliptically polarized laser fields within a minimal three-state electronic model under the frozen-nuclei approximation. However, that approach did not address the preparation of appropriate initial conditions or the tailored light\u2013matter interactions required to create photon-dressed states. To overcome this limitation, it is crucial to consider a process that prepares the photon-dressed states from the electronic ground state through optical pumping with pulsed lasers. In this work, we analytically design such pulsed lasers to induce helical photon-dressed states in both low- and high-symmetry aromatic rings, starting from the ground state. We further incorporate the nuclear vibrational effects within the adiabatic approximation and apply those designed laser fields to low-symmetry aromatic rings. Finally, we numerically demonstrate the generation of angular momenta associated with the photon-dressed states using the analytically designed laser fields. Vibrational effects are found to selectively influence the stability of specific photon-dressed states.<\/jats:p>","DOI":"10.1063\/5.0315624","type":"journal-article","created":{"date-parts":[[2026,4,8]],"date-time":"2026-04-08T10:38:12Z","timestamp":1775644692000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":0,"title":["Theoretical quantum design of pump-laser pulses for generating helical photon-dressed states"],"prefix":"10.1063","volume":"164","author":[{"ORCID":"https:\/\/orcid.org\/0009-0004-3720-9606","authenticated-orcid":false,"given":"Quang Huy","family":"Ho","sequence":"first","affiliation":[{"name":"Faculty of Engineering Technology, University of Phan Thiet 1 , 225 Nguyen Thong, Phu Thuy, Lam Dong,","place":["Vietnam"]},{"name":"Nuclear Training Center, VINATOM 2 , Hanoi 10000,","place":["Vietnam"]}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2292-6157","authenticated-orcid":false,"given":"Ngoc Loan","family":"Phan","sequence":"additional","affiliation":[{"name":"Computational Physics Laboratory K002, Department of Physics, Ho Chi Minh City University of Education 3 , Ho Chi Minh City,","place":["Vietnam"]}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4835-6634","authenticated-orcid":false,"given":"Hirobumi","family":"Mineo","sequence":"additional","affiliation":[{"name":"Atomic Molecular and Optical Physics Research Group, Science and Technology Advanced Institute, Van Lang University 4 , Ho Chi Minh City,","place":["Vietnam"]},{"name":"Faculty of Applied Technology, Van Lang School of Technology, Van Lang University 5 , Ho Chi Minh City,","place":["Vietnam"]}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"317","published-online":{"date-parts":[[2026,4,8]]},"reference":[{"key":"2026040806380712400_c1","doi-asserted-by":"publisher","first-page":"144310","DOI":"10.1063\/1.2185633","article-title":"Optimal control of ultrafast laser driven many-electron dynamics in a polyatomic molecule: N-methyl-6-quinolone","volume":"124","year":"2006","journal-title":"J.\u00a0Chem. 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