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Dielectric spectroscopy can be used to probe whether the collective reorientation of the hydrogen-bonding superstructure has timescales associated with methanol and water separately or a single relaxation, indicating a hybrid structure. Through analysis of the component spectra, we find only one relaxation accounting for all hydrogen-bonding structure reorientations across the entire composition range, indicating that a hybrid hydrogen bonding structure is indeed formed across that entire range.<\/jats:p>","DOI":"10.1063\/5.0320783","type":"journal-article","created":{"date-parts":[[2026,3,2]],"date-time":"2026-03-02T14:27:48Z","timestamp":1772461668000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":3,"title":["Computational dielectric spectroscopy shows that water\/methanol mixtures form hybrid hydrogen bonding networks"],"prefix":"10.1063","volume":"164","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-4743-8475","authenticated-orcid":false,"given":"Rebecca A.","family":"Bone","sequence":"first","affiliation":[{"name":"Theiss Research 1 , P.O. 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