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While experiments are advancing toward the realization of chiral cavities, a mean-field theoretical framework for describing electron\u2013photon interaction in this platform has been missing. Here, we present a mean-field theory that can be systematically improved to capture the chiral correlation effects responsible for the enantioselective power of chiral light. We use strong coupling M\u00f8ller\u2013Plesset perturbation theory for accessing the excitation manifold of electrons and chiral virtual photons. We apply the developed methods to selected chiral systems and show that the mean-field theory captures cavity frequency dispersion but fails to describe the chiral discrimination arising from coupled electron\u2013photon excitations.<\/jats:p>","DOI":"10.1063\/5.0333560","type":"journal-article","created":{"date-parts":[[2026,7,16]],"date-time":"2026-07-16T10:58:00Z","timestamp":1784199480000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":0,"title":["Unveiling chiral electron\u2013photon correlation effects in circularly polarized optical devices"],"prefix":"10.1063","volume":"165","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-4551-7188","authenticated-orcid":false,"given":"Yassir","family":"El Moutaoukal","sequence":"first","affiliation":[{"name":"Department of Chemistry, Norwegian University of Science and Technology 1 , 7491 Trondheim,","place":["Norway"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6870-4237","authenticated-orcid":false,"given":"Rosario R.","family":"Riso","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Norwegian University of Science and Technology 1 , 7491 Trondheim,","place":["Norway"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0000-1713-0635","authenticated-orcid":false,"given":"Andrea","family":"Bianchi","sequence":"additional","affiliation":[{"name":"Scuola Normale Superiore 2 , Piazza dei Cavalieri 7, 56126 Pisa, PI,","place":["Italy"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8367-8727","authenticated-orcid":false,"given":"Henrik","family":"Koch","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Norwegian University of Science and Technology 1 , 7491 Trondheim,","place":["Norway"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"317","published-online":{"date-parts":[[2026,7,16]]},"reference":[{"key":"2026071606575116200_c1","doi-asserted-by":"publisher","first-page":"2766","DOI":"10.1039\/d4cc05598e","article-title":"Optical cavity enhancement of visible light-driven photochemical reaction in the crystalline state","volume":"61","year":"2025","journal-title":"Chem. 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