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We recorded the optical spectrum of gas-phase AuC between 400 and 700\u00a0nm, assigning excitations from the X2\u03a01\/2((2\u03c3)2(2\u03c0)1) ground state to states arising from the (2\u03c3)2(3\u03c3*)1 and (2\u03c3)1(2\u03c0)2 configurations. Dispersed-fluorescence spectra are used to study the vibrational and spin\u2013orbit structure of the ground state, branching ratios and radiative lifetimes of the excited states, and the Au\u2013C bond dissociation energy. A molecular orbital diagram is used to rationalize the nature of AuC\u2019s low-lying electronic states. The data serve as valuable benchmarks of relativistic theory and are relevant to quantum science and precision measurements with cold molecules.<\/jats:p>","DOI":"10.1063\/5.0337427","type":"journal-article","created":{"date-parts":[[2026,6,8]],"date-time":"2026-06-08T10:57:55Z","timestamp":1780916275000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":0,"title":["Elucidating Au\u2013C bonding via laser spectroscopy of gold monocarbide"],"prefix":"10.1063","volume":"164","author":[{"ORCID":"https:\/\/orcid.org\/0009-0005-0149-9565","authenticated-orcid":false,"given":"Rory M.","family":"Weldon","sequence":"first","affiliation":[{"name":"Department of Chemistry, Williams College , Williamstown, Massachusetts 01267,","place":["USA"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Danielle M.","family":"Darling","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Williams College , Williamstown, Massachusetts 01267,","place":["USA"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-6440-519X","authenticated-orcid":false,"given":"Nicole M.","family":"Albright","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Williams College , Williamstown, Massachusetts 01267,","place":["USA"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0009-4580-863X","authenticated-orcid":false,"given":"Kendall L.","family":"Rice","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Williams College , Williamstown, Massachusetts 01267,","place":["USA"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Phaedra L.","family":"Salerno","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Williams College , Williamstown, Massachusetts 01267,","place":["USA"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0004-2624-5863","authenticated-orcid":false,"given":"K. 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