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Nevertheless, the puzzling ascendancy of spin in the oxygen evolution reaction (OER) process remains an enigma owing to the robust correlation between TM 4d and oxygen 2p orbitals. Herein, we employed SrRuO3 (SRO) with 4d electron states as a ferromagnetic catalyst for the OER, which were deposited onto the flexible mica substrates. By applying compressive or tensile stresses to the SRO film, the bipolar enhancement of OER activity was observed. At the potential of 1.8\u00a0V, the current density (j) of SRO enhanced by \u223c34% or \u223c44%, with a 0.2% compressive or tensile strain, respectively, attributing to the diminished chemisorption of Ru\u2013O. In addition, it was found that j enhanced by \u223c86% or \u223c104% and the overpotential reduced by \u223c20% or \u223c26% at a 0.2% compressive or tensile strain with a 13 kOe in-plane (IP) magnetic field, respectively. Those were attributing to the enhancement of the double exchange effect and the concentration of O22\u2212 in SRO, thus promoting electron transfer and regulating the adsorption\/desorption capacity of reaction intermediates, respectively. Moreover, the magnetohydrodynamic-induced bubble effect is one of the factors that enhance the electrocatalytic activity. This investigation offers experimental evidence to comprehend the regulation of spin degree and electronic state during OER, hence advancing the design and engineering of the flexible magnetoelectrochemistry catalysts with encouraging prospects.<\/jats:p>","DOI":"10.1063\/5.0345139","type":"journal-article","created":{"date-parts":[[2026,8,6]],"date-time":"2026-08-06T15:52:11Z","timestamp":1786031531000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":0,"title":["Enhanced oxygen evolution reaction via the tunability of spin and electronic states in a flexible van der Waals membranous catalyst"],"prefix":"10.1063","volume":"165","author":[{"given":"Hang","family":"Xu","sequence":"first","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mi","family":"Du","sequence":"additional","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu","family":"Liu","sequence":"additional","affiliation":[{"name":"China Germanium Co., Ltd. 2 , Nanjing 211200,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Linglong","family":"Hu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]},{"name":"Jilin Key Laboratory of Solid Laser Technology and Application, College of Science, Changchun University of Science and Technology 3 , Changchun 130022,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Daming","family":"Yang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chaoqun","family":"Qu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zeyu","family":"Zhao","sequence":"additional","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5921-0190","authenticated-orcid":false,"given":"Ming","family":"Feng","sequence":"additional","affiliation":[{"name":"Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University 1 , Changchun 130103,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"317","published-online":{"date-parts":[[2026,8,6]]},"reference":[{"key":"2026080611520854300_c1","doi-asserted-by":"publisher","first-page":"1378","DOI":"10.1038\/s41467-020-15231-x","article-title":"Cation insertion to break the activity\/stability relationship for highly active oxygen evolution reaction catalyst","volume":"11","year":"2020","journal-title":"Nat. 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