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In this work, we develop a comprehensive Brownian dynamics framework to compute the frequency-dependent admittance of nanocapacitors, explicitly accounting for salt concentration and the finite screening length of electrodes (modeled via Thomas\u2013Fermi theory). We derive the fluctuation\u2013dissipation relation connecting the dynamics of equilibrium charge fluctuations to the linear response of the system quantified by the frequency-dependent admittance. In particular, we obtain two estimators for the admittance\u2014based on ionic positions and forces\u2014and combine them via a control variate method to reduce statistical uncertainty across all frequencies. Our simulations show that the admittance exhibits a low-frequency regime dominated by capacitive effects and a high-frequency one governed by the ideal Nernst\u2013Einstein conductivity. The crossover between these regimes is characterized by a timescale that depends on both the electrode metallicity and salt concentration, highlighting the role of ion\u2013wall collisions and electrostatic interactions. Comparisons with analytical models show that while mean-field theories capture qualitative trends, they systematically overestimate low-frequency admittance and underestimate high-frequency behavior, underscoring the necessity of explicit ion\u2013ion and ion\u2013wall interactions. This work connects microscopic dynamics to macroscopic electrochemical observables, offering a tool to interpret impedance spectra in nanoscale systems. Beyond charge storage in EDLCs, our framework provides insights for sensing applications in nanofluidic devices, where charge\/current fluctuations enable the detection of electrochemically active species.<\/jats:p>","DOI":"10.1063\/5.0350617","type":"journal-article","created":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T10:39:44Z","timestamp":1791196784000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":0,"title":["Dynamics of charge fluctuations in nanocapacitors: Effects of salt concentration and electrode metallicity from Brownian dynamics"],"prefix":"10.1063","volume":"165","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-7257-8125","authenticated-orcid":false,"given":"Paul","family":"Desmarchelier","sequence":"first","affiliation":[{"name":"Sorbonne Universit\u00e9, CNRS, Laboratoire PHENIX (Physicochimie des \u00c9lectrolytes et Nanosyst\u00e8mes Interfaciaux) 1 , 4 Place Jussieu, 75005 Paris,","place":["France"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5198-4650","authenticated-orcid":false,"given":"Benjamin","family":"Rotenberg","sequence":"additional","affiliation":[{"name":"Sorbonne Universit\u00e9, CNRS, Laboratoire PHENIX (Physicochimie des \u00c9lectrolytes et Nanosyst\u00e8mes Interfaciaux) 1 , 4 Place Jussieu, 75005 Paris,","place":["France"]},{"name":"R\u00e9seau sur le Stockage \u00c9lectrochimique de l\u2019\u00c9nergie (RS2E), FR CNRS 3459 2 , 80039 Amiens Cedex,","place":["France"]}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"317","published-online":{"date-parts":[[2026,10,5]]},"reference":[{"key":"2026100506393912200_c1","doi-asserted-by":"publisher","first-page":"813","DOI":"10.1021\/cr00103a008","volume":"90","year":"1990","journal-title":"Chem. 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