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To demonstrate the capabilities of this method, they implemented it in a real-space (basis-set-free) code and applied it to benchmark molecules, namely, CO, H2O, and para-nitroaniline. Their results are in agreement with experimental and previous theoretical studies and fully validate their approach.<\/jats:p>","DOI":"10.1063\/1.2733666","type":"journal-article","created":{"date-parts":[[2007,5,11]],"date-time":"2007-05-11T16:23:53Z","timestamp":1178900633000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":110,"title":["Time-dependent density functional theory scheme for efficient calculations of dynamic (hyper)polarizabilities"],"prefix":"10.1063","volume":"126","author":[{"given":"Xavier","family":"Andrade","sequence":"first","affiliation":[{"name":"UPV\/EHU Departamento de F\u00edsica de Materiales, Facultad de Ciencias Qu\u00edmicas, Centro Mixto and European Theoretical Spectroscopy Facility (ETSF), E\u201320018 San Sebasti\u00e1n, Spain; Laboratoire des Solides Irradi\u00e9s, CNRS-CEA-\u00c9cole Polytechnique, F-91128 Palaiseau, France"},{"name":"CSIC-UPV\/EHU Departamento de F\u00edsica de Materiales, Facultad de Ciencias Qu\u00edmicas, Centro Mixto and European Theoretical Spectroscopy Facility (ETSF), E\u201320018 San Sebasti\u00e1n, Spain; Laboratoire des Solides Irradi\u00e9s, CNRS-CEA-\u00c9cole Polytechnique, F-91128 Palaiseau, France"}]},{"given":"Silvana","family":"Botti","sequence":"additional","affiliation":[{"name":"Universidade de Coimbra Laboratoire des Solides Irradi\u00e9s, CNRS-CEA-\u00c9cole Polytechnique and European Theoretical Spectroscopy Facility (ETSF), F-91128, France; and Centro de F\u00edsica Computacional, Departamento de F\u00edsica, , P-3004516 Coimbra, Portugal"}]},{"given":"Miguel A. 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