{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2025,7,30]],"date-time":"2025-07-30T11:14:01Z","timestamp":1753874041953,"version":"3.41.2"},"reference-count":44,"publisher":"AIP Publishing","issue":"1","funder":[{"DOI":"10.13039\/501100002347","name":"Bundesministerium f\u00fcr Bildung und Forschung","doi-asserted-by":"publisher","award":["05K16PGA","05K16SI1"],"award-info":[{"award-number":["05K16PGA","05K16SI1"]}],"id":[{"id":"10.13039\/501100002347","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/100010661","name":"Horizon 2020 Framework Programme","doi-asserted-by":"publisher","award":["654002"],"award-info":[{"award-number":["654002"]}],"id":[{"id":"10.13039\/100010661","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001871","name":"Funda\u00e7\u00e3o para a Ci\u00eancia e a Tecnologia","doi-asserted-by":"publisher","award":["CERN-FIS-PAR-0005-2017"],"award-info":[{"award-number":["CERN-FIS-PAR-0005-2017"]}],"id":[{"id":"10.13039\/501100001871","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["pubs.aip.org"],"crossmark-restriction":true},"short-container-title":[],"published-print":{"date-parts":[[2019,7,7]]},"abstract":"<jats:p>In the current work, we present an investigation of the electronic and defect structure in (TiO2) rutile monocrystals by virtue of time differential perturbed angular \u03b3-\u03b3 correlation spectroscopy. Studies were performed using 111mCd, implanted at ISOLDE\/CERN complemented with diffusion studies and density functional theory calculations. Hyperfine field parameters have been probed as a function of temperature between 298\u2009K and 873\u2009K. The results demonstrate that 111mCd\/Cd implanted rutile has two local environments. The first environment is characterized with parameters attributed to Cd localized at the cationic site which goes relatively along with a specific case where a charged supercell Cd:Ti(2e\u2212) is in the scope. The origin of the second fraction could be rising from the subsurface regions where according to a tracer diffusion study the major part of implant is bounded featuring different diffusion mechanisms. Performed ab initio calculations suggest that the disruptive surface environment could contain apical or equatorial vacancies near the probe, inducing high electric field gradients for the second fraction. Current results seem to differ from those obtained before with different methods of probing (Ag\/Cd and In\/Cd).<\/jats:p>","DOI":"10.1063\/1.5102134","type":"journal-article","created":{"date-parts":[[2019,7,2]],"date-time":"2019-07-02T14:53:25Z","timestamp":1562079205000},"update-policy":"https:\/\/doi.org\/10.1063\/aip-crossmark-policy-page","source":"Crossref","is-referenced-by-count":4,"title":["Hyperfine interactions and diffusion of Cd in TiO2 (rutile)"],"prefix":"10.1063","volume":"126","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3834-7555","authenticated-orcid":false,"given":"Dmitry V.","family":"Zyabkin","sequence":"first","affiliation":[{"name":"Chair Materials for Electrical Engineering and Electronics, Institute of Materials Science and Engineering, Institute of Micro and Nanotechnologies MacroNano\u00ae, TU Ilmenau 1 , Gustav-Kirchhoff-Strasse 5, 98693 Ilmenau, Germany"},{"name":"Department of Experimental Physics, Faculty of Science, Palack\u00fd University in Olomouc 2 , 17. Listopadu 12, 77147 Olomouc, Czechia"}]},{"given":"Juliana","family":"Schell","sequence":"additional","affiliation":[{"name":"Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen 3 , 45141 Essen, Germany"},{"name":"European Organization for Nuclear Research (CERN) 4 , CH-1211 Geneva, Switzerland"}]},{"given":"Daniel","family":"Gaertner","sequence":"additional","affiliation":[{"name":"Institute of Materials Physics, University of M\u00fcnster 5 , D-48149 M\u00fcnster, Germany"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9633-5654","authenticated-orcid":false,"given":"Thanh T.","family":"Dang","sequence":"additional","affiliation":[{"name":"University of Bonn 6 Helmholtz-Institut f\u00fcr Strahlen- und Kernphysik, , 53115 Bonn, Germany"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9057-378X","authenticated-orcid":false,"given":"Jo\u00e3o N.","family":"Gon\u00e7alves","sequence":"additional","affiliation":[{"name":"Departmento de F\u00edsica and CICECO, Universidade de Aveiro 7 , 3810-193 Aveiro, Portugal"}]},{"given":"Georg","family":"Marschick","sequence":"additional","affiliation":[{"name":"Vienna University of Technology 8 , 1040 Vienna, Austria"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8802-6621","authenticated-orcid":false,"given":"Peter","family":"Schaaf","sequence":"additional","affiliation":[{"name":"Chair Materials for Electrical Engineering and Electronics, Institute of Materials Science and Engineering, Institute of Micro and Nanotechnologies MacroNano\u00ae, TU Ilmenau 1 , Gustav-Kirchhoff-Strasse 5, 98693 Ilmenau, Germany"}]}],"member":"317","published-online":{"date-parts":[[2019,7,2]]},"reference":[{"key":"2023062321512394900_c1","doi-asserted-by":"publisher","first-page":"103","DOI":"10.1016\/j.mssp.2015.03.032","volume":"36","year":"2015","journal-title":"Mater. 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