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Phys.: Condens. Matter"],"published-print":{"date-parts":[[2024,10,23]]},"abstract":"<jats:title>Abstract<\/jats:title>\n               <jats:p>Spin\u2013orbit coupling offers a large variety of novel and extraordinary magnetic and electronic properties in otherwise \u2018ordinary pool\u2019 of heavy ion oxides. Here we present a detailed study on an apparently isolated hexagonal 2<jats:italic>H<\/jats:italic> spin-chain <jats:italic>d<\/jats:italic>\n                  <jats:sup>4<\/jats:sup> iridate Sr<jats:sub>3<\/jats:sub>LiIrO<jats:sub>6<\/jats:sub> with geometric frustration. Our structural studies reveal Li\u2013Ir chemical order with desired stoichiometry in this compound, while x-ray absorption together with x-ray photoemission spectroscopic characterizations establish pure 5+ valence of Ir. We have established a magnetic ground state with finite Ir<jats:sup>5+<\/jats:sup> magnetic moments in this compound, contrary to the anticipated nonmagnetic <jats:inline-formula>\n                     <jats:tex-math\/>\n                     <mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\" overflow=\"scroll\">\n                        <mml:mrow>\n                           <mml:msub>\n                              <mml:mi>J<\/mml:mi>\n                              <mml:mrow>\n                                 <mml:mrow>\n                                    <mml:mi>eff<\/mml:mi>\n                                 <\/mml:mrow>\n                              <\/mml:mrow>\n                           <\/mml:msub>\n                        <\/mml:mrow>\n                     <\/mml:math>\n                  <\/jats:inline-formula> = 0 state, through combined dc susceptibility, <jats:inline-formula>\n                     <jats:tex-math\/>\n                     <mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\" overflow=\"scroll\">\n                        <mml:mrow>\n                           <mml:msup>\n                              <mml:mrow\/>\n                              <mml:mn>7<\/mml:mn>\n                           <\/mml:msup>\n                        <\/mml:mrow>\n                     <\/mml:math>\n                  <\/jats:inline-formula>Li nuclear magnetic resonance (NMR), muon spin relaxation (<jats:italic>\u00b5<\/jats:italic>SR) and <jats:italic>ab-initio<\/jats:italic> electronic structure studies. These investigations together with ac magnetic susceptibility and specific heat measurements reveal that despite having noticeable antiferromagnetic correlation among the Ir<jats:sup>5+<\/jats:sup> local moments, this system does not magnetically order down to at least 0.05 K, possibly due to geometrical exchange frustration, arising from the comparable nearest- and next-nearest-neighbor interchain Ir\u2013O\u2013O\u2013Ir superexchange interaction strengths with opposite signs. However, the zero-field <jats:italic>\u00b5<\/jats:italic>SR analysis shows emergence of a considerable proportion of spin-freezing on top of a spin-fluctuating dynamic magnetic background down to the lowest measured temperature of 1.7\u2009K, possibly due to some inhomogeneity and\/or the much stronger intra-column Ir\u2013Ir magnetic exchange interaction strength relative to the inter-column Ir\u2013Ir ones. The linear temperature dependence of the magnetic specific heat (<jats:inline-formula>\n                     <jats:tex-math\/>\n                     <mml:math xmlns:mml=\"http:\/\/www.w3.org\/1998\/Math\/MathML\" overflow=\"scroll\">\n                        <mml:mrow>\n                           <mml:msub>\n                              <mml:mi>C<\/mml:mi>\n                              <mml:mrow>\n                                 <mml:mi mathvariant=\"normal\">m<\/mml:mi>\n                              <\/mml:mrow>\n                           <\/mml:msub>\n                        <\/mml:mrow>\n                     <\/mml:math>\n                  <\/jats:inline-formula>) in both zero and applied magnetic fields, plus the power-law behavior of the NMR spin-lattice relaxation rate suggest a gapless spinon density of states in this charge gapped disordered magnetic ground state of Sr<jats:sub>3<\/jats:sub>LiIrO<jats:sub>6<\/jats:sub>.<\/jats:p>","DOI":"10.1088\/1361-648x\/ad63eb","type":"journal-article","created":{"date-parts":[[2024,7,16]],"date-time":"2024-07-16T22:55:57Z","timestamp":1721170557000},"page":"425804","update-policy":"https:\/\/doi.org\/10.1088\/crossmark-policy","source":"Crossref","is-referenced-by-count":1,"title":["Disordered magnetic ground state in a quasi-1-D d\n               <sup>4<\/sup> columnar iridate Sr<sub>3<\/sub>LiIrO<sub>6<\/sub>"],"prefix":"10.1088","volume":"36","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-9332-8985","authenticated-orcid":true,"given":"Abhisek","family":"Bandyopadhyay","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Debu","family":"Das","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"A","family":"Chakraborty","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"S","family":"Bhowal","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Vinod","family":"Kumar","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"G B G","family":"Stenning","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3674-3378","authenticated-orcid":true,"given":"C","family":"Ritter","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2280-079X","authenticated-orcid":true,"given":"D T","family":"Adroja","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"M","family":"Moretti Sala","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"A","family":"Efimenko","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4846-8422","authenticated-orcid":true,"given":"C","family":"Meneghini","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"F","family":"Bert","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7367-5960","authenticated-orcid":true,"given":"P K","family":"Biswas","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6012-9530","authenticated-orcid":true,"given":"I","family":"Dasgupta","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"T","family":"Saha Dasgupta","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"A V","family":"Mahajan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7180-1241","authenticated-orcid":true,"given":"Sugata","family":"Ray","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"266","published-online":{"date-parts":[[2024,7,25]]},"reference":[{"key":"cmad63ebbib1","doi-asserted-by":"publisher","DOI":"10.1088\/0034-4885\/80\/1\/016502","volume":"80","author":"Savary","year":"2017","journal-title":"Rep. 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