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No significant structural distortion from cubic symmetry <jats:italic>Fd-<\/jats:italic>3m was noticed for all the compositions in the range 0 \u2a7d <jats:italic>x<\/jats:italic>\u2a7d 1 of Ni(Cr<jats:sub>1\u2212<jats:italic>x<\/jats:italic>\n                  <\/jats:sub>Mn<jats:italic>\n                     <jats:sub>x<\/jats:sub>\n                  <\/jats:italic>)<jats:sub>2<\/jats:sub>O<jats:sub>4<\/jats:sub>. However, there is significant alteration in the bond angles <jats:italic>\u2220<\/jats:italic>B<jats:italic>\u2013<\/jats:italic>O<jats:italic>\u2013<\/jats:italic>B (90.51\u00b0-93.86\u00b0) and <jats:italic>\u2220<\/jats:italic>A<jats:italic>\u2013<\/jats:italic>O<jats:italic>\u2013<\/jats:italic>B (122.48\u00b0\u2013124.90\u00b0) (both of which follow completely opposite trend with increasing <jats:italic>x<\/jats:italic>) and bond lengths A<jats:italic>\u2013<\/jats:italic>O (1.82\u20131.94 \u00c5) and B<jats:italic>\u2013<\/jats:italic>O (2.02\u20132.08 \u00c5). The corresponding lattice parameter (<jats:italic>a<\/jats:italic>) follows Vegard\u2019s law (8.32 \u00b1 0.001 \u00c5 \u2a7d <jats:italic>a<\/jats:italic> \u2a7d 8.45 \u00b1 0.001\u00c5). The electronic structure determined from the <jats:italic>x-<\/jats:italic>ray photoelectron spectroscopy reveals the divalent nature of Ni (with spin\u2013orbit splitting energy \u0394 \u223c 17.62 eV). While the Cr and Mn are stable with trivalent electronic states having \u0394 <jats:italic>=<\/jats:italic>8 and 11.7 eV, respectively. These results are in consonance with the cationic distribution (Ni)<jats:sub>A<\/jats:sub>[(Cr<jats:sub>1\u2212<jats:italic>x<\/jats:italic>\n                  <\/jats:sub>Mn<jats:italic>\n                     <jats:sub>x<\/jats:sub>\n                  <\/jats:italic>)<jats:sub>2<\/jats:sub>]<jats:sub>B<\/jats:sub>O<jats:sub>4<\/jats:sub> obtained from the Rietveld refinement analysis. Interestingly, the current series shows a direct bandgap (<jats:italic>E<\/jats:italic>\n                  <jats:sub>G<\/jats:sub>) semiconducting nature in which <jats:italic>E<\/jats:italic>\n                  <jats:sub>G<\/jats:sub> varies from 1.16 to 2.40 eV within the range of <jats:italic>x<\/jats:italic> = 0.85\u20130. Such variation of <jats:italic>E<\/jats:italic>\n                  <jats:sub>G<\/jats:sub> (<jats:italic>x<\/jats:italic>) is consistent with the compositional variation of the crystal structure data with anomalous change between <jats:italic>x<\/jats:italic> = 0.25 and 0.6. Beyond this range, the <jats:italic>E<\/jats:italic>\n                  <jats:sub>g<\/jats:sub> mode (140 cm<jats:sup>\u22121<\/jats:sup>) in Raman spectra arising from Mn\u2013O octahedral decreases continuously and vanishes at higher Mn concentrations. Our analysis shows that all the investigated compounds show long-range ferrimagnetic ordering below the N\u00e9el temperature, <jats:italic>T<\/jats:italic>\n                  <jats:sub>FN<\/jats:sub> due to the unequal magnetic moments of the cations. However, both the ordering temperature <jats:italic>T<\/jats:italic>\n                  <jats:sub>FN<\/jats:sub> and saturation magnetization (<jats:italic>M<\/jats:italic>\n                  <jats:sub>S<\/jats:sub>) increases progressively from 73.3 K (1500 emu mol<jats:sup>\u22121<\/jats:sup>) to 116 K (3600 emu mol<jats:sup>\u22121<\/jats:sup>) with increasing the Mn content from 0 to 1, yet the maximum anisotropy (<jats:italic>H<jats:sub>K<\/jats:sub>\n                  <\/jats:italic>~4.5 kOe, <jats:italic>K<\/jats:italic>\n                  <jats:sub>1<\/jats:sub>~2.5 \u00d7 10<jats:sup>4<\/jats:sup> erg cc<jats:sup>\u22121<\/jats:sup>) shows an opposite trend with <jats:italic>x<\/jats:italic>. Such variation is ascribed to the altered magnetic superexchange interactions between the cations located at A and B sites following the trend <jats:italic>J<\/jats:italic>\n                  <jats:sub>BB<\/jats:sub> &gt; <jats:italic>J<\/jats:italic>\n                  <jats:sub>AB<\/jats:sub> &gt; <jats:italic>J<\/jats:italic>\n                  <jats:sub>AA<\/jats:sub>, (<jats:italic>J<\/jats:italic>\n                  <jats:sub>BB<\/jats:sub>\/<jats:italic>k<\/jats:italic>\n                  <jats:sub>B<\/jats:sub> =13.36 K).<\/jats:p>","DOI":"10.1088\/1361-648x\/ad9537","type":"journal-article","created":{"date-parts":[[2024,11,21]],"date-time":"2024-11-21T13:11:08Z","timestamp":1732194668000},"page":"075402","update-policy":"https:\/\/doi.org\/10.1088\/crossmark-policy","source":"Crossref","is-referenced-by-count":2,"title":["Evolution of tunable energy bandgap and magnetic anisotropy in Mn substituted ferrimagnetic nickel-chromates"],"prefix":"10.1088","volume":"37","author":[{"ORCID":"https:\/\/orcid.org\/0009-0007-4074-5436","authenticated-orcid":false,"given":"A","family":"Datta","sequence":"first","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4754-2504","authenticated-orcid":false,"given":"T","family":"Sarkar","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9128-5563","authenticated-orcid":true,"given":"M","family":"Roy-Chowdhury","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6352-1167","authenticated-orcid":false,"given":"P","family":"Tiwari","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9326-6323","authenticated-orcid":true,"given":"H","family":"Singh","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0965-1486","authenticated-orcid":true,"given":"J K","family":"Dey","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0740-2195","authenticated-orcid":true,"given":"S","family":"Thota","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"266","published-online":{"date-parts":[[2024,12,3]]},"reference":[{"key":"cmad9537bib1","doi-asserted-by":"publisher","first-page":"1","DOI":"10.1016\/j.physrep.2021.04.002","volume":"926","author":"Tsurkan","year":"2021","journal-title":"Phys. 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