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In the rigid limit, amorphous regions reemerge and expand, and high-density systems fail to crystallize completely, instead forming mixed phases with HCP-like and disordered local environments. This transition arises from geometric frustration: rigid dimers are unable to adjust their internal configuration to optimize local packing, thereby suppressing crystallization and promoting amorphization. Our findings reveal that bond flexibility is a key control parameter governing structural organization in core\u2013softened colloidal and molecular systems, offering insights for the design of tunable soft materials.<\/jats:p>","DOI":"10.1088\/1361-648x\/ae170f","type":"journal-article","created":{"date-parts":[[2025,10,23]],"date-time":"2025-10-23T22:55:21Z","timestamp":1761260121000},"page":"445101","update-policy":"https:\/\/doi.org\/10.1088\/crossmark-policy","source":"Crossref","is-referenced-by-count":3,"title":["How soft is too soft? 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