{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T14:17:35Z","timestamp":1788963455330,"version":"build-2803163510"},"reference-count":86,"publisher":"IOP Publishing","issue":"36","license":[{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/publishingsupport.iopscience.iop.org\/iop-standard\/v1"},{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"tdm","delay-in-days":0,"URL":"https:\/\/iopscience.iop.org\/info\/page\/text-and-data-mining"},{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/publishingsupport.iopscience.iop.org\/questions\/alternative-author-rights-policies\/"},{"start":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:00:00Z","timestamp":1788912000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/publishingsupport.iopscience.iop.org\/questions\/alternative-author-rights-policies\/"}],"funder":[{"name":"UGC-DAE CSR, Mumbai","award":["CRS\/2021-22\/03\/576"],"award-info":[{"award-number":["CRS\/2021-22\/03\/576"]}]},{"name":"University Grant Commission"}],"content-domain":{"domain":["iopscience.iop.org"],"crossmark-restriction":false},"short-container-title":["J. Phys.: Condens. Matter"],"published-print":{"date-parts":[[2026,9,11]]},"abstract":"Abstract<\/jats:title>\n \n Here, we report an interesting magnetic oxide Na\n \n \n \n <\/jats:tex-math>\n \n \n \n \n 3<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n Ni\n \n \n \n <\/jats:tex-math>\n \n \n \n \n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n SbO\n \n \n \n <\/jats:tex-math>\n \n \n \n \n 6<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n , where the interplay between exchange interactions and lattice symmetry crucially influence its exotic ground state (GS). This compound features a layered honeycomb lattice with magnetic Ni\n \n \n \n <\/jats:tex-math>\n \n \n \n \n \n 2<\/mml:mn>\n +<\/mml:mo>\n <\/mml:mrow>\n <\/mml:msup>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n (spin-1) surrounding nonmagnetic Sb\n \n \n \n <\/jats:tex-math>\n \n \n \n \n \n 5<\/mml:mn>\n +<\/mml:mo>\n <\/mml:mrow>\n <\/mml:msup>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n centers. The x-ray absorption and magnetic circular dichroism measurements confirm a Ni\n \n \n \n <\/jats:tex-math>\n \n \n \n \n \n 2<\/mml:mn>\n +<\/mml:mo>\n <\/mml:mrow>\n <\/mml:msup>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n charge state with notable spin and orbital moments at room temperature. The material exhibits antiferromagnetic (AFM) ordering around 17 K (\n \n \n \n <\/jats:tex-math>\n \n \n \n T<\/mml:mi>\n N<\/mml:mi>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n ) and a field-induced magnetic transition at lower temperatures. Our measurements reveal a low-temperature anomaly, likely linked to glassy behavior. The power-law magnetic specific heat suggests mixed magnon dispersion, while low magnetic entropy indicates a highly degenerate GS. Neutron diffraction data point to a zigzag-type AFM GS, with a reduced site moment of 1.34(3)\n \n \n \n <\/jats:tex-math>\n \n \n \n \u03bc<\/mml:mi>\n \n B<\/mml:mi>\n <\/mml:mrow>\n <\/mml:msub>\n \n \/<\/mml:mo>\n <\/mml:mrow>\n \n \n Ni<\/mml:mi>\n <\/mml:mrow>\n \n 2<\/mml:mn>\n +<\/mml:mo>\n <\/mml:mrow>\n <\/mml:msup>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n at 2.5 K that disappears near 17.2 K, consistent with bulk data. Lattice parameters show anomalies at\n \n \n \n <\/jats:tex-math>\n \n \n \n T<\/mml:mi>\n N<\/mml:mi>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n and lower temperatures. Ab-initio calculations support zigzag spin order and imply a competing in-plane Ni\n \n \n \n <\/jats:tex-math>\n \n \n \n \n \n 2<\/mml:mn>\n +<\/mml:mo>\n <\/mml:mrow>\n <\/mml:msup>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n interactions that causes spin frustration. Overall, our combined experimental and theoretical study uncovers the microscopic magnetic GS of Na\n \n \n \n <\/jats:tex-math>\n \n \n \n \n 3<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n Ni\n \n \n \n <\/jats:tex-math>\n \n \n \n \n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n SbO\n \n \n \n <\/jats:tex-math>\n \n \n \n \n 6<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n as a mix of long-range zigzag AFM and a glassy state, advancing the understanding of frustrated honeycomb magnets.\n <\/jats:p>","DOI":"10.1088\/1361-648x\/ae9fa7","type":"journal-article","created":{"date-parts":[[2026,8,27]],"date-time":"2026-08-27T22:53:33Z","timestamp":1787871213000},"page":"365801","update-policy":"https:\/\/doi.org\/10.1088\/crossmark-policy","source":"Crossref","is-referenced-by-count":0,"title":["Coexisting long-range zigzag antiferromagnetic order and glassy dynamics in spin-1 honeycomb lattice Na\n 3<\/sub>\n Ni\n 2<\/sub>\n SbO\n 6<\/sub>"],"prefix":"10.1088","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-0299-6708","authenticated-orcid":true,"given":"R K","family":"Patel","sequence":"first","affiliation":[{"name":"Jawaharlal Nehru University"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0406-5947","authenticated-orcid":true,"given":"B","family":"Saha","sequence":"additional","affiliation":[{"name":"Bhabha Atomic Research Centre"},{"name":"Homi Bhabha National Institute"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Debashish","family":"Das","sequence":"additional","affiliation":[{"name":"Indian Institute of Technology"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0222-0990","authenticated-orcid":false,"given":"A K","family":"Bera","sequence":"additional","affiliation":[{"name":"Bhabha Atomic Research Centre"},{"name":"Homi Bhabha National Institute"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kranti","family":"Kumar","sequence":"additional","affiliation":[{"name":"UGC-DAE Consortium for Scientific Research"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4361-294X","authenticated-orcid":true,"given":"Chandrani","family":"Nath","sequence":"additional","affiliation":[{"name":"Jawaharlal Nehru University"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0001-3574-9623","authenticated-orcid":true,"given":"V R","family":"Singh","sequence":"additional","affiliation":[{"name":"Central University of South Bihar"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kenta","family":"Amemiya","sequence":"additional","affiliation":[{"name":"Tsukuba"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0613-219X","authenticated-orcid":true,"given":"K","family":"Asokan","sequence":"additional","affiliation":[{"name":"Inter-University Accelerator Centre"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1898-4610","authenticated-orcid":true,"given":"S M","family":"Yusuf","sequence":"additional","affiliation":[{"name":"Bhabha Atomic Research Centre"},{"name":"Homi Bhabha National Institute"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"M P","family":"Saravanan","sequence":"additional","affiliation":[{"name":"UGC-DAE Consortium for Scientific Research"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8458-1006","authenticated-orcid":true,"given":"Aftab","family":"Alam","sequence":"additional","affiliation":[{"name":"Indian Institute of Technology Bombay"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9354-8395","authenticated-orcid":true,"given":"A K","family":"Pramanik","sequence":"additional","affiliation":[{"name":"Jawaharlal Nehru University"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"266","published-online":{"date-parts":[[2026,9,9]]},"reference":[{"key":"cmae9fa7bib1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.86.144404","type":"journal-article","article-title":"Phase diagram of a frustrated Heisenberg antiferromagnet on the honeycomb lattice: The J1- J2- J3 model","volume":"86","author":"Li","year":"2012","journal-title":"Phys. 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