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Herein, we report a novel catalytic introduction method of graphene with adjustable porosity by high-energy photon beam. The graphene\/Ti\n                    <jats:sub>3<\/jats:sub>\n                    C\n                    <jats:sub>2<\/jats:sub>\n                    T\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    heterostructure was constructed by electrostatic self-assembly, has a high cycle life (98% after 8000 cycles), energy density (11.02 mWh cm\n                    <jats:sup>\u22123<\/jats:sup>\n                    ), and demonstrate excellent flexible alternating current line-filtering performance. The phase angle of \u221279.8\u00b0 at 120 Hz and a resistance-capacitance constant of 0.068 ms. Furthermore, the porous graphene\/Ti\n                    <jats:sub>3<\/jats:sub>\n                    C\n                    <jats:sub>2<\/jats:sub>\n                    T\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    structures produced by multiple catalytic inductions allowed ions to deeply penetrate the electrode, thereby increasing the stacking density. The special \u2018pore-layer nesting\u2019 graphene structure with adjustable pores effectively increased the specific surface area, and its superior matching with electrolyte solutions greatly improved surface-active site utilization. This work offers an alternative strategy for fabricating a 2D heterostructure for an MSC.\n                  <\/jats:p>","DOI":"10.1088\/1361-6528\/ad64de","type":"journal-article","created":{"date-parts":[[2024,7,18]],"date-time":"2024-07-18T18:48:56Z","timestamp":1721328536000},"page":"425401","update-policy":"https:\/\/doi.org\/10.1088\/crossmark-policy","source":"Crossref","is-referenced-by-count":5,"title":["Photon-beam-inducing synthesis of a tunable porous graphene\/Ti\n                    <sub>3<\/sub>\n                    C\n                    <sub>2<\/sub>\n                    T\n                    <i>\n                      <sub>x<\/sub>\n                    <\/i>\n                    heterostructure for energy conversion-storage system"],"prefix":"10.1088","volume":"35","author":[{"given":"Maoyang","family":"Xia","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qianqian","family":"Liu","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3766-1158","authenticated-orcid":true,"given":"Jing","family":"Ning","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1686-4068","authenticated-orcid":true,"given":"Dong","family":"Wang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Hao","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jincheng","family":"Zhang","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"266","published-online":{"date-parts":[[2024,7,29]]},"reference":[{"key":"nanoad64debib1","doi-asserted-by":"publisher","first-page":"266","DOI":"10.1016\/j.nanoen.2018.01.004","article-title":"MXene electrochemical microsupercapacitor integrated with triboelectric nanogenerator as a wearable self-charging power unit","volume":"45","author":"Jiang","year":"2018","journal-title":"Nano Energy"},{"key":"nanoad64debib2","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2020.104741","article-title":"Functional integrated electromagnetic interference shielding in flexible micro-supercapacitors by cation-intercalation typed Ti3C2Tx MXene","volume":"72","author":"Feng","year":"2020","journal-title":"Nano Energy"},{"key":"nanoad64debib3","doi-asserted-by":"publisher","first-page":"844","DOI":"10.1038\/s41578-022-00508-y","article-title":"Sustainable flexible supercapacitors","volume":"7","author":"Pacchioni","year":"2022","journal-title":"Nat. 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