{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,3,31]],"date-time":"2026-03-31T22:34:24Z","timestamp":1774996464798,"version":"3.50.1"},"reference-count":128,"publisher":"IOP Publishing","issue":"8","license":[{"start":{"date-parts":[[2023,8,8]],"date-time":"2023-08-08T00:00:00Z","timestamp":1691452800000},"content-version":"vor","delay-in-days":7,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0"},{"start":{"date-parts":[[2023,8,8]],"date-time":"2023-08-08T00:00:00Z","timestamp":1691452800000},"content-version":"tdm","delay-in-days":7,"URL":"https:\/\/iopscience.iop.org\/info\/page\/text-and-data-mining"}],"funder":[{"name":"European Union\u2019s Horizon 2020","award":["MSCA ITN 813393"],"award-info":[{"award-number":["MSCA ITN 813393"]}]},{"DOI":"10.13039\/501100023561","name":"Spanish Ministerio de Universidades","doi-asserted-by":"crossref","id":[{"id":"10.13039\/501100023561","id-type":"DOI","asserted-by":"crossref"}]},{"name":"Funda\u00e7\u00e3o para a Ci\u00eancia e a Tecnologia","award":["EXPL\/FIS-PLA\/0076\/2021"],"award-info":[{"award-number":["EXPL\/FIS-PLA\/0076\/2021"]}]},{"DOI":"10.13039\/501100000780","name":"European Union","doi-asserted-by":"crossref","id":[{"id":"10.13039\/501100000780","id-type":"DOI","asserted-by":"crossref"}]}],"content-domain":{"domain":["iopscience.iop.org"],"crossmark-restriction":false},"short-container-title":["Plasma Sources Sci. Technol."],"published-print":{"date-parts":[[2023,8,1]]},"abstract":"Abstract<\/jats:title>\n This work presents a reaction mechanism for oxygen plasmas, i.e. a set of reactions and corresponding rate coefficients that are validated against benchmark experiments. The kinetic scheme is validated in a DC glow discharge for gas pressures of 0.2\u201310\u2009Torr and currents of 10\u201340\u2009mA, using the 0D LisbOn KInetics simulation tool and available experimental data. The comparison comprises not only the densities of the main species in the discharge\u2014\n \n \n \n \n O<\/mml:mi>\n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n (<\/mml:mo>\n \n \n X<\/mml:mi>\n <\/mml:mrow>\n 3<\/mml:mn>\n <\/mml:msup>\n \n \u0394<\/mml:mi>\n \n g<\/mml:mi>\n <\/mml:mrow>\n \u2212<\/mml:mo>\n <\/mml:msubsup>\n )<\/mml:mo>\n <\/mml:math>\n \n <\/jats:inline-formula>, \n \n \n \n \n O<\/mml:mi>\n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n (<\/mml:mo>\n \n \n a<\/mml:mi>\n 1<\/mml:mn>\n <\/mml:msup>\n <\/mml:mrow>\n \n \u0394<\/mml:mi>\n \n g<\/mml:mi>\n <\/mml:mrow>\n <\/mml:msub>\n )<\/mml:mo>\n <\/mml:math>\n \n <\/jats:inline-formula>, \n \n \n \n \n O<\/mml:mi>\n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n (<\/mml:mo>\n \n \n b<\/mml:mi>\n 1<\/mml:mn>\n <\/mml:msup>\n <\/mml:mrow>\n \n \u03a3<\/mml:mi>\n \n \n g<\/mml:mi>\n +<\/mml:mo>\n <\/mml:msup>\n <\/mml:mrow>\n <\/mml:msub>\n )<\/mml:mo>\n <\/mml:math>\n \n <\/jats:inline-formula> and \n \n \n \n O<\/mml:mi>\n \n \n (<\/mml:mo>\n 3<\/mml:mn>\n <\/mml:msup>\n <\/mml:mrow>\n P<\/mml:mi>\n )<\/mml:mo>\n <\/mml:mrow>\n <\/mml:math>\n \n <\/jats:inline-formula>\u2014but also the self-consistent calculation of the reduced electric field and the gas temperature. The main processes involved in the creation and destruction of these species are identified. Moreover, the results show that the oxygen atoms play a dominant role in gas heating, via recombination at the wall and quenching of \n \n \n \n \n O<\/mml:mi>\n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n (<\/mml:mo>\n \n \n X<\/mml:mi>\n <\/mml:mrow>\n 3<\/mml:mn>\n <\/mml:msup>\n \n \u03a3<\/mml:mi>\n \n \n g<\/mml:mi>\n \u2212<\/mml:mo>\n <\/mml:msup>\n ,<\/mml:mo>\n v<\/mml:mi>\n <\/mml:mrow>\n <\/mml:msub>\n )<\/mml:mo>\n <\/mml:math>\n \n <\/jats:inline-formula> vibrations and \n \n \n \n \n O<\/mml:mi>\n 2<\/mml:mn>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n \n <\/jats:inline-formula> electronically-excited states. It is argued that the development and validation of kinetic schemes for plasma chemistry should adopt a paradigm based on the comparison against standard validation tests<\/jats:italic>, as it is done in electron swarm validation of cross sections.<\/jats:p>","DOI":"10.1088\/1361-6595\/aceaa4","type":"journal-article","created":{"date-parts":[[2023,7,26]],"date-time":"2023-07-26T22:28:51Z","timestamp":1690410531000},"page":"084003","update-policy":"https:\/\/doi.org\/10.1088\/crossmark-policy","source":"Crossref","is-referenced-by-count":34,"title":["A reaction mechanism for oxygen plasmas"],"prefix":"10.1088","volume":"32","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-2179-1345","authenticated-orcid":true,"given":"Tiago C","family":"Dias","sequence":"first","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8230-2322","authenticated-orcid":true,"given":"Chlo\u00e9","family":"Fromentin","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2677-574X","authenticated-orcid":false,"given":"Lu\u00eds L","family":"Alves","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9147-7909","authenticated-orcid":true,"given":"Antonio","family":"Tejero-del-Caz","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9046-958X","authenticated-orcid":true,"given":"Tiago","family":"Silva","sequence":"additional","affiliation":[]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6878-6850","authenticated-orcid":true,"given":"Vasco","family":"Guerra","sequence":"additional","affiliation":[]}],"member":"266","published-online":{"date-parts":[[2023,8,8]]},"reference":[{"key":"psstaceaa4bib1","doi-asserted-by":"publisher","first-page":"236","DOI":"10.1109\/TPS.2005.845345","article-title":"Selective oxygen plasma etching of coatings","volume":"33","author":"Cvelbar","year":"2005","journal-title":"IEEE Trans. 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