{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,11,1]],"date-time":"2026-11-01T03:16:24Z","timestamp":1793502984500,"version":"4.5.0"},"reference-count":53,"publisher":"Oxford University Press (OUP)","issue":"1","license":[{"start":{"date-parts":[[2025,10,17]],"date-time":"2025-10-17T00:00:00Z","timestamp":1760659200000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["42025706"],"award-info":[{"award-number":["42025706"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52270015"],"award-info":[{"award-number":["52270015"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"name":"China National Postdoctoral Program for Innovative Talents","award":["BX20250326"],"award-info":[{"award-number":["BX20250326"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,1,10]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>Insufficient charge separation and sluggish two-electron water-oxidation reaction are two critical factors restricting the photosynthesis performance of metal-free covalent organic frameworks (COFs) for hydrogen peroxide (H2O2) generation from naturally abundant water and air. Herein, we develop a facile strategy to simultaneously boost the charge-separation efficiency and water-oxidation capability through constructing short and rapid charge-transfer tunnels within highly charge-confined COFs via replacing the phenyl with pyrimidine. Compared with a single charge-transfer tunnel within a lowly charge-confined COF-5-(4-aminophenyl)pyrimidin-2-amine (APM) with pyrimidine, dual charge-transfer tunnels are constructed within a highly charge-confined COF-5,5\u2032-bipyrimidine-2,2\u2032-diamine (BPM) with bipyrimidine due to the ground-state charge transfer between para-carbon and meta-nitrogen, which significantly accelerates the intermolecular charge-transfer process and prevents charge recombination. This strategy also decreases the energy barrier of rate-determining water oxidation in H2O2 photosynthesis and thus promotes the effective generation of the key *OH intermediates, facilitating the generation of H2O2 at a production rate of 5521 \u03bcmol g\u22121 h\u22121 from water, oxygen and light without sacrificial reagents or additional energy consumption by COF-BPM. Furthermore, COF-BPM can also efficiently produce H2O2 under broad pH conditions, in widely available real water, on a floatable foam sheet, in a continuous-flow reactor and in a scaled-up reactor by using natural solar light for water decontamination.<\/jats:p>","DOI":"10.1093\/nsr\/nwaf444","type":"journal-article","created":{"date-parts":[[2025,10,16]],"date-time":"2025-10-16T12:15:09Z","timestamp":1760616909000},"source":"Crossref","is-referenced-by-count":3,"title":["Constructing dual charge-transfer tunnels within highly charge-confined COFs for efficient photosynthesis of hydrogen peroxide from water and air"],"prefix":"10.1093","volume":"13","author":[{"given":"Yanghui","family":"Hou","sequence":"first","affiliation":[{"name":"College of Environmental Sciences and Engineering, Peking University , Beijing 100871 ,","place":["China"]},{"name":"The Key Laboratory of Water and Sediment Sciences (Ministry of Education), Peking University , Beijing 100871 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Sediment Sciences (Ministry of Education), Peking University , Beijing 100871 ,","place":["China"]},{"name":"State Environmental Protection Key Laboratory of All Material Fluxes in River Ecosystems, Peking University , Beijing 100871 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jialiang","family":"Liang","sequence":"additional","affiliation":[{"name":"College of Environment and Ecology, Chongqing University , Chongqing 400045 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peng","family":"Zhou","sequence":"additional","affiliation":[{"name":"Eco-environment and Resource Efficiency Research Laboratory, School of Environment and Energy, Peking University Shenzhen Graduate School , Shenzhen 518055 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Meiping","family":"Tong","sequence":"additional","affiliation":[{"name":"College of Environmental Sciences and Engineering, Peking 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