{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,27]],"date-time":"2026-10-27T22:02:27Z","timestamp":1793138547652,"version":"4.5.0"},"reference-count":56,"publisher":"Oxford University Press (OUP)","issue":"4","license":[{"start":{"date-parts":[[2026,1,10]],"date-time":"2026-01-10T00:00:00Z","timestamp":1768003200000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["U21A20174"],"award-info":[{"award-number":["U21A20174"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/100012541","name":"Guangdong Innovative and Entrepreneurial Research Team Program","doi-asserted-by":"publisher","award":["2021ZT09L197"],"award-info":[{"award-number":["2021ZT09L197"]}],"id":[{"id":"10.13039\/100012541","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,2,5]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>Direct recycling has emerged as a promising alternative to existing recycling methods due to its simplicity and cost-effectiveness. However, its scalable application remains a subject of debate, primarily due to the complexity of mixed degraded cathode materials in practice. The reason is that degraded materials with different compositions are extremely difficult to be repaired to produce cathode materials with uniform composition and performance. Herein, we have successfully realized direct regeneration of mixed heterogeneous degraded LiNi0.5Co0.2Mn0.3O2 from different sources on an industrial scale. First, uniform contact lithiation is achieved through the van der Waals force between Li-1-methyl-2-pyrrolidinone and LiNi0.5Co0.2Mn0.3O2 molecules, leaving them in a uniform lithium-rich state. A self-saturating synthetic lithiation process occurs during subsequent heating, ensuring that each particle from various sources is repaired as needed. This method has been demonstrated to treat 50\u00a0kg of cathode materials per batch, and the regenerated products show uniform and excellent performance, achieving a retention rate of 90.7% after 1500 cycles in Ah-level pouch cells. This performance is the best result reported to date and sets a new benchmark for regenerated LiNixCoyMn1-x-yO2 cathode materials, which have reached the standard for direct commercial use.<\/jats:p>","DOI":"10.1093\/nsr\/nwag017","type":"journal-article","created":{"date-parts":[[2026,1,10]],"date-time":"2026-01-10T12:37:17Z","timestamp":1768048637000},"source":"Crossref","is-referenced-by-count":16,"title":["Flexible direct regeneration of heterogeneous cathode materials of spent lithium-ion batteries at industrial scale"],"prefix":"10.1093","volume":"13","author":[{"given":"Junxiong","family":"Wang","sequence":"first","affiliation":[{"name":"Tsinghua Shenzhen International Graduate School, Tsinghua University , Shenzhen 518055 ,","place":["China"]},{"name":"Frontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University , Shanghai 200240 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