{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,11,2]],"date-time":"2026-11-02T23:03:54Z","timestamp":1793660634518,"version":"4.5.1"},"reference-count":49,"publisher":"Oxford University Press (OUP)","issue":"10","license":[{"start":{"date-parts":[[2026,3,10]],"date-time":"2026-03-10T00:00:00Z","timestamp":1773100800000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/100022964","name":"Key Research and Development Program of Zhejiang Province","doi-asserted-by":"publisher","award":["2024C03112"],"award-info":[{"award-number":["2024C03112"]}],"id":[{"id":"10.13039\/100022964","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/100022964","name":"Key Research and Development Program of Zhejiang Province","doi-asserted-by":"publisher","award":["2024C03128"],"award-info":[{"award-number":["2024C03128"]}],"id":[{"id":"10.13039\/100022964","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100017623","name":"Zhejiang Provincial Outstanding Youth Science Foundation","doi-asserted-by":"publisher","award":["LR26B070001"],"award-info":[{"award-number":["LR26B070001"]}],"id":[{"id":"10.13039\/501100017623","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22376183"],"award-info":[{"award-number":["22376183"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,5,21]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>Efficiently utilizing carbon resources from waste plastics and expanding pathways for high-value chemical production are crucial for sustainable development and advancing the circular economy. However, the challenge of inert and hard-to-reuse CO2 released during plastic management remains a significant hurdle, resulting in the loss of valuable carbon resources. Herein, we propose a versatile in situ CO2-capturing strategy for the efficient upcycling of polycarbonate (PC) to produce bisphenol A (BPA) and diverse CO2-upgraded products. Utilizing a variety of CO2-capturing reagents, including nitriles, epoxies, amines, alkynes and alcohols, we achieve complete depolymerization of PC under mild, atmospheric conditions and efficiently co-produce value-added chemicals such as nitrogen-containing heterocycles, cyclic carbonates and acetylenic carboxylic acids. Mechanistic studies reveal that the process involves a more thermodynamically favorable in situ CO2 capture pathway compared to conventional gaseous CO2. This strategy offers a new route to unlock carbon resources from carbonate-based polymers for diversified chemical production and sustainable waste management.<\/jats:p>","DOI":"10.1093\/nsr\/nwag153","type":"journal-article","created":{"date-parts":[[2026,3,10]],"date-time":"2026-03-10T12:35:05Z","timestamp":1773146105000},"source":"Crossref","is-referenced-by-count":3,"title":["<i>In situ<\/i>\n                    CO2 capture: a general strategy for valorizing waste polycarbonate into high-value chemicals"],"prefix":"10.1093","volume":"13","author":[{"given":"Minghao","family":"Zhang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Soil Pollution Control and Safety, Zhejiang University , Hangzhou 310058 ,","place":["China"]},{"name":"College of Environmental and Resource Sciences, Zhejiang University , Hangzhou 310058 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,","place":["China"]},{"name":"College of Environmental and Resource Sciences, Zhejiang University , Hangzhou 310058 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zexiang","family":"Wu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Soil Pollution Control and Safety, Zhejiang University , Hangzhou 310058 ,","place":["China"]},{"name":"College of Environmental and Resource Sciences, Zhejiang University , Hangzhou 310058 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weixiang","family":"Wu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Soil Pollution Control and Safety, Zhejiang University , Hangzhou 310058 ,","place":["China"]},{"name":"College of Environmental and Resource Sciences, Zhejiang University , Hangzhou 310058 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