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However, a challenge encountered by these non-conjugated structures is that the fluorescence of pure hydrocarbon systems is largely confined to the blue region (\u223c470\u00a0nm), raising the question of whether this is a fundamental limitation. Herein, we break this barrier by constructing a library of over 50 non-conjugated arylated alkenes via binuclear nickel-catalyzed hydroarylation of allenes. It is disclosed that synergistic multiple through-space interactions (TSIs) including molecular twisting-tuned intramolecular TSIs combined with intermolecular TSIs mediated by the double bonds of styrene units are critical for achieving the ultralong-wavelength aggregation-induced emission of these non-conjugated structures. This enables tunable light emission from blue to yellow, orange and, remarkably, even to single-compound-based warm white light. Furthermore, strategic substitution extends the fluorescence into the deep-red region, with a tail reaching 900\u00a0nm. This work demonstrates that non-conjugated pure hydrocarbons can achieve a broad spectrum of colors, fundamentally advancing the understanding of the luminescence phenomenon of non-conjugated systems and providing a novel design strategy for luminescent materials beyond the traditional TBC paradigm.<\/jats:p>","DOI":"10.1093\/nsr\/nwag257","type":"journal-article","created":{"date-parts":[[2026,5,6]],"date-time":"2026-05-06T11:41:39Z","timestamp":1778067699000},"source":"Crossref","is-referenced-by-count":2,"title":["Breaking the blue limit of non-conjugated hydrocarbons via multiple through-space interactions"],"prefix":"10.1093","volume":"13","author":[{"ORCID":"https:\/\/orcid.org\/0009-0004-4741-3766","authenticated-orcid":false,"given":"Shuxin","family":"Jiang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Organometallic Chemistry and Shanghai-Hong Kong Joint Laboratory in Chemical Synthesis, Shanghai Institute of Organic Chemistry, University of Chinese 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