{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,28]],"date-time":"2026-10-28T16:52:31Z","timestamp":1793206351308,"version":"4.5.0"},"reference-count":51,"publisher":"Oxford University Press (OUP)","issue":"15","license":[{"start":{"date-parts":[[2026,5,23]],"date-time":"2026-05-23T00:00:00Z","timestamp":1779494400000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2022YFA1504700"],"award-info":[{"award-number":["2022YFA1504700"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22308266"],"award-info":[{"award-number":["22308266"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["U21A20317"],"award-info":[{"award-number":["U21A20317"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["U23A20132"],"award-info":[{"award-number":["U23A20132"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,8,10]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>CO2 catalytic hydrogenation presents a highly promising and alternative pathway for ethanol production, offering the dual benefits of large-scale CO2 emission reduction and green H2 storage. However, this approach faces major challenges such as low ethanol selectivity and activity, stemming from the complex reaction network and the lack of efficient catalyst design strategies. In this work, we proposed an effective catalyst design strategy for CO2 hydrogenation to ethanol by constructing synergetic catalytic sites between alloy nanoparticles and zeolite to decouple key competing reaction steps. The developed PdCu alloy catalyst encapsulated by Y zeolite achieved simultaneously high ethanol selectivity (&amp;gt;93%) and activity (&amp;gt;200\u00a0mg gcat\u22121 h\u22121), outperforming most previously reported heterogeneous catalysts. Mechanistic investigations revealed that the alloy\u2013zeolite synergetic sites facilitate controllable C\u2013C coupling and enhance C\u2013O bond cleavage, thereby balancing selectivity and catalytic activity toward CO2 hydrogenation to ethanol. This work offers a feasible catalyst design strategy for the efficient conversion of CO2 into high-value-added and structurally complex products.<\/jats:p>","DOI":"10.1093\/nsr\/nwag303","type":"journal-article","created":{"date-parts":[[2026,5,22]],"date-time":"2026-05-22T11:51:34Z","timestamp":1779450694000},"source":"Crossref","is-referenced-by-count":2,"title":["Synergetic catalysis via zeolite-encapsulated PdCu alloy for highly efficient CO2 hydrogenation to ethanol"],"prefix":"10.1093","volume":"13","author":[{"given":"Di","family":"Xu","sequence":"first","affiliation":[{"name":"School of Power and Mechanical Engineering, Wuhan University , Wuhan 430072 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaojia","family":"Song","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Clean and Efficient Coal Utilization, College of Chemistry and Chemical Engineering, Taiyuan University of Technology , Taiyuan 030024 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