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Progress has been limited by inefficient synthesis-and-testing cycles and the lack of simple design rules linking molecular structure to excited-state relaxation. Here, we establish a predictive design framework for ultranarrow multiple-resonance emitters by treating molecular topology as an explicit handle on structural relaxation. High-throughput screening of B,N-doped triangulene fusion modes identifies an alternating fusion pattern that minimizes reorganization energy and yields a ground-state descriptor for spectral narrowing without explicit excited-state calculations. Guided by this framework, we synthesize sky-blue emitters with photoluminescence bandwidths down to 9.1\u00a0nm and solution-processed devices with 10.9-nm electroluminescence bandwidths and 38.1% external quantum efficiency.<\/jats:p>","DOI":"10.1093\/nsr\/nwag377","type":"journal-article","created":{"date-parts":[[2026,6,20]],"date-time":"2026-06-20T11:37:47Z","timestamp":1781955467000},"source":"Crossref","is-referenced-by-count":14,"title":["Molecular-topology-guided multiple-resonance emitters with sub-10-nm bandwidths: ultranarrow high-efficiency solution-processable OLEDs"],"prefix":"10.1093","volume":"13","author":[{"given":"Tao","family":"Hua","sequence":"first","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 ,","place":["China"]},{"name":"Institute of Technology for Future Industry, School of Science and Technology Instrument Application Engineering, Shenzhen University of Information Technology , Shenzhen 518172 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nengquan","family":"Li","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 ,","place":["China"]},{"name":"Institute of Technology for Future Industry, School of Science and Technology Instrument Application Engineering, Shenzhen University of Information Technology , Shenzhen 518172 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaosong","family":"Cao","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Cheng","family":"Zhong","sequence":"additional","affiliation":[{"name":"College of Chemistry and Molecular Sciences, Wuhan University , Wuhan 430072 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingsheng","family":"Miao","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhongyan","family":"Huang","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 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,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Youming","family":"Zhang","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 ,","place":["China"]},{"name":"Institute of Technology for Future Industry, School of Science and Technology Instrument Application Engineering, Shenzhen University of Information Technology , Shenzhen 518172 ,","place":["China"]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chuluo","family":"Yang","sequence":"additional","affiliation":[{"name":"Shenzhen Key Laboratory of New Information Display and Storage Materials, College of Materials Science and Engineering, Shenzhen University , Shenzhen 518060 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