{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,30]],"date-time":"2026-09-30T03:53:11Z","timestamp":1790740391398,"version":"4.1.0"},"reference-count":55,"publisher":"Oxford University Press (OUP)","issue":"18","license":[{"start":{"date-parts":[[2026,6,25]],"date-time":"2026-06-25T00:00:00Z","timestamp":1782345600000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22579141"],"award-info":[{"award-number":["22579141"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22379125"],"award-info":[{"award-number":["22379125"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["20720250114"],"award-info":[{"award-number":["20720250114"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":[],"published-print":{"date-parts":[[2026,9,21]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>Aqueous zinc-bromine (Zn-Br2) batteries are promising candidates for grid-scale energy storage owing to their low cost and inherent safety. However, their areal capacity and cycling stability are severely limited by detrimental polybromide shuttling, which arises from concentration-gradient-driven diffusion and often overlooked internal-electric-field-accelerated electromigration. Herein, a bulk-to-interphase synergistic regulation strategy is proposed integrating electrostatic micropore confinement in the cathode bulk with additional interfacial anchoring and electric-field-responsive recovery at the cathode\/electrolyte interphase. Poly(quaternary ammonium)-functionalized activated carbon (N+-AC) hosts are rationally designed to trap polybromide anions within positively charged micropores of cathode bulk, thereby suppressing concentration-gradient-driven leakage while maintaining fast conversion kinetics. Simultaneously, 1-butyl-3-methylimidazolium chloride (1,3-MI) electrolyte additive adsorbed on the cathode surface provides additional polybromide anchoring at the interphase. Importantly, theoretical calculations and in situ characterizations demonstrate that an electric-field-responsive 1,3-MI accumulation layer forms spontaneously during discharge, dynamically attracting polybromides and inhibiting their electromigration toward the anode, thus promoting their recovery to the cathode for reversible redox conversion. Consequently, the N+-AC||Zn full cell with 1,3-MI achieves stable cycling over 1000 cycles at an ultrahigh areal capacity of 10 mAh cm\u22122. Furthermore, Ah-level Zn-Br2 pouch cells operate stably at both room and subzero temperatures, validating the practical potential of this electric-field-aware bulk-to-interphase regulation strategy under complex climatic conditions.<\/jats:p>","DOI":"10.1093\/nsr\/nwag393","type":"journal-article","created":{"date-parts":[[2026,6,24]],"date-time":"2026-06-24T11:56:21Z","timestamp":1782302181000},"source":"Crossref","is-referenced-by-count":2,"title":["Bulk-to-interphase polybromide confinement and electric-field-responsive recovery enable Ah-level aqueous zinc-bromine batteries at room\/low temperatures"],"prefix":"10.1093","volume":"13","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-5069-1455","authenticated-orcid":false,"given":"Qilong","family":"Wu","sequence":"first","affiliation":[{"name":"State Key Laboratory of Physical Chemistry of Solid Surfaces, State-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, College of Chemistry and Chemical 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