{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,6]],"date-time":"2026-10-06T04:08:13Z","timestamp":1791259693425,"version":"4.1.0"},"reference-count":37,"publisher":"The Royal Society","issue":"9","license":[{"start":{"date-parts":[[2024,9,1]],"date-time":"2024-09-01T00:00:00Z","timestamp":1725148800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"},{"start":{"date-parts":[[2024,9,1]],"date-time":"2024-09-01T00:00:00Z","timestamp":1725148800000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"content-domain":{"domain":["royalsocietypublishing.org"],"crossmark-restriction":true},"short-container-title":["R. Soc. Open Sci."],"published-print":{"date-parts":[[2024,9]]},"abstract":"<jats:p>\n            This study aimed to investigate the catalytic performance of H-ZSM-5 zeolite compared with physically mixed and sequentially used synthesized \u03b3-alumina and zeolite in the methanol-to-propylene (MTP) reaction. A facile, green and cost-effective method was first applied to prepare a mesoporous \u03b3-Al\n            <jats:sub>2<\/jats:sub>\n            O\n            <jats:sub>3<\/jats:sub>\n            support using a combination of sol\u2013gel and hydrothermal methods via a few consecutive steps. This process was carried out using aluminium nitrate and polyethylene glycol with different molecular weights as non-ionic surfactants. X-ray diffraction, transmission electon microscopy, thermogravimetric analysis, ammonia temperature programmed desorption and Brunauer\u2013Emmett\u2013Teller analysis were then used to characterize the prepared \u03b3-Al\n            <jats:sub>2<\/jats:sub>\n            O\n            <jats:sub>3<\/jats:sub>\n            catalyst. Afterwards, the catalytic activity of the commercial H-ZSM-5 zeolite (Si\/Al = 200) and the effect of the presence of the \u03b3-alumina physically mixed and unmixed with the zeolite were also researched in the MTP reaction. Accordingly, methanol conversion and product selectivity were monitored via gas chromatography. The physically mixed mesoporous \u03b3-Al\n            <jats:sub>2<\/jats:sub>\n            O\n            <jats:sub>3<\/jats:sub>\n            and H-ZSM-5 zeolite exhibited the highest catalytic activity in terms of both conversion and selectivity at 400\u00b0C. To our knowledge, this research represents the first documented use of \u03b3-alumina and zeolite simultaneously as catalysts in the MTP reaction within the English literature. It is hoped that this work will offer valuable insights for advancing the development of catalytic systems in methanol conversion processes.\n          <\/jats:p>","DOI":"10.1098\/rsos.240469","type":"journal-article","created":{"date-parts":[[2024,9,18]],"date-time":"2024-09-18T07:32:11Z","timestamp":1726644731000},"update-policy":"https:\/\/doi.org\/10.1098\/crossmark-policy","source":"Crossref","is-referenced-by-count":1,"title":["Comparative study of the catalytic performance of physically mixed and sequentially utilized \u03b3-alumina and zeolite in methanol-to-propylene reactions"],"prefix":"10.1098","volume":"11","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-1502-2371","authenticated-orcid":true,"given":"Anahita","family":"Mortazavi-Manesh","sequence":"first","affiliation":[{"name":"Department of Chemistry, Faculty of Chemistry and Petroleum Science, Shahid Beheshti University, GC , Tehran 1983969411, Iran"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8286-0415","authenticated-orcid":true,"given":"Nasser","family":"Safari","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Faculty of Chemistry and Petroleum Science, Shahid Beheshti University, GC , Tehran 1983969411, Iran"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mojtaba","family":"Golbodaqi","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Faculty of Chemistry and Petroleum Science, Shahid Beheshti University, GC , Tehran 1983969411, Iran"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shirin","family":"Latifi","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Faculty of Chemistry and Petroleum Science, Shahid Beheshti University, GC , Tehran 1983969411, Iran"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mohammad","family":"Fatehi Haghighat","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Faculty of Chemistry and Petroleum Science, Shahid Beheshti University, GC , Tehran 1983969411, Iran"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Farzad","family":"Bahadoran","sequence":"additional","affiliation":[{"name":"Gas Research Division, Research Institute of Petroleum Industry (RIPI) , Tehran 1485733111, Iran"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"175","published-online":{"date-parts":[[2024,9,18]]},"reference":[{"key":"e_1_3_8_2_2","doi-asserted-by":"crossref","first-page":"8888","DOI":"10.1021\/acs.iecr.7b01967","article-title":"Preparation of large-pore-volume \u03b3-alumina nanofibers with a narrow pore size distribution in a membrane dispersion microreactor","volume":"56","author":"Wan Y","year":"2017","unstructured":"Wan Y , Liu Y , Wang Y , Luo G . 2017 Preparation of large-pore-volume \u03b3-alumina nanofibers with a narrow pore size distribution in a membrane dispersion microreactor. 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